Crystal material, preparation method and application thereof, battery positive electrode active material, battery positive electrode material, battery and electric equipment
A technology of crystalline materials and battery positive electrodes, which is applied in the direction of battery electrodes, secondary batteries, carboxylate preparations, etc., can solve the problems of unsatisfactory electrochemical performance of potassium ion batteries and limited types of positive electrode active materials, so as to reduce the preparation cost, Raw materials are cheap and the effect of increasing battery capacity
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[0051] According to a second aspect of the present invention, the present invention provides a method for preparing a crystalline material, comprising the steps of:
[0052] Solvothermal reaction of potassium source, lithium source, transition metal source and oxalic acid source to obtain KLi 3 Tm(C 2 o 4 ) 3 , Tm is a transition metal;
[0053] Wherein, the transition metal source is selected from cobalt source, nickel source, manganese source, copper source, zinc source, titanium source, vanadium source
[0054] The preparation method of the crystal material provided by the present invention adopts low-cost potassium source, lithium source, transition metal source and oxalic acid source to prepare through solvothermal reaction, the process is simple, the operation is convenient, and the cost of the positive active material of the battery can be effectively reduced. application prospects.
[0055] In a preferred embodiment of the present invention, the temperature of the...
Embodiment 1
[0150] This embodiment provides a KLi 3 Co(C 2 o 4 ) 3 Crystal material, its preparation method comprises the steps:
[0151] 0.23793g CoCl 2 ·6H 2 O, 0.14778g Li 2 CO 3 , 0.13821g K 2 CO 3 , 0.50428g H 2 C 2 o 4 2H 2 O, 10g H 2 O was put into a 25mL polytetrafluoroethylene inner village hydrothermal reaction kettle, stirred and mixed evenly, the reaction kettle was tightened, put into an oven at 190°C, reacted for 4 hours and cooled to room temperature, the solid product in the reaction kettle was taken out, cleaned, Suction filtration, obtain KLi after drying 3 Co(C 2 o 4 ) 3 crystal particles.
Embodiment 2
[0153] This embodiment provides a KLi 3 Co(C 2 o 4 ) 3 Crystalline material, the difference between its preparation method and embodiment 1 is that K 2 CO 3 It is 0.22642g.
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