Phenolic resin microspheres with concave-convex structure and preparation method thereof
A technology of phenolic resin and concave-convex structure, applied in the field of concave-convex structure phenolic resin microspheres and its preparation, can solve the problems of difficult waste disposal and high processing costs, and achieve easy activation to form pores, high carbonization yield, and excellent thermal stability Effect
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[0024] According to another aspect of the present application, there is provided a method for preparing the concave-convex structure phenolic resin microspheres, at least comprising the following steps:
[0025] 1) dissolving the thermoplastic phenolic resin in an alkaline solution to obtain an alkaline phenolic resin solution A;
[0026] 2) Mixing the phenolic resin acidic waste water with the solution A, heating and reacting;
[0027] 3) After separation and drying, the phenolic resin microspheres are obtained.
[0028] Further, the thermoplastic phenolic resin can be a phenolic resin familiar to those skilled in the art, such as phenol-formaldehyde resin, resorcinol-formaldehyde resin, 3-aminophenol-formaldehyde resin, bisphenol A-formaldehyde resin or various modified Resins, including but not limited to one or more of cardanol modified phenolic resin, boron modified phenolic resin, silicon modified phenolic resin, selenium modified phenolic resin.
[0029] Further, the ...
Embodiment 1
[0040] Thermoplastic phenol-formaldehyde resin 2g is dissolved in 50ml aqueous sodium hydroxide solution to obtain alkaline phenolic resin solution; 50g phenolic resin acidic wastewater (pH is 2.3, phenol content is 2512mg / L, aldehyde content is 5548mg / L, COD is 38546mg / L.) mixed with alkaline phenolic resin solution, adjusted to pH 8.5, heated to 100°C for 8 hours; centrifuged at 5000r / min for 5min, then dried in an oven at 120°C to obtain phenolic resin microspheres. The prepared phenolic phenolic resin microspheres have an average particle size of 268nm and a surface specific surface area of 48m 2 / g, please refer to figure 1 .
[0041] Wherein, the microsphere specific surface area is physical adsorption specific surface area, which can be obtained according to GB / T19587-2004 gas adsorption BET method, the surface specific surface area is calculated by t-Plot method, and the average particle size is tested by laser particle size analyzer.
Embodiment 2
[0043] Thermoplastic phenol-formaldehyde resin 2g is dissolved in 50ml aqueous sodium hydroxide solution to obtain alkaline phenolic resin solution; 95g phenolic resin acidic wastewater (pH is 1.8, phenol content is 965mg / L, aldehyde content is 4560mg / L, COD is 18322mg / L.) mixed with alkaline phenolic resin solution, adjusted to pH 8.0, heated to 100°C for 12h; separated by a centrifuge at 5000r / min for 5min, then dried in an oven at 120°C to obtain phenolic resin microspheres. The prepared phenolic phenolic resin microspheres have an average particle size of 186nm and a surface specific surface area of 51m 2 / g.
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