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Silicon carbide fiber material with rare earth modified lanthanum phosphate coating, and preparation method and application thereof

A technology of silicon carbide fiber and rare earth modification, applied in the field of inorganic non-metallic surface treatment, can solve problems such as performance degradation and SiC fiber degradation, achieve wide application prospects and overcome the effect of degradation performance degradation

Inactive Publication Date: 2020-12-25
GUANGDONG INST OF NEW MATERIALS
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

However, related studies have found that in high-temperature reducing atmospheres with LaPO 4 Coated SiC fibers degrade and degrade performance, which limits LaPO 4 Application of coating in non-oxide ceramic matrix composite system

Method used

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Experimental program
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preparation example Construction

[0031] Further, in order to further improve the 4 The physical properties and oxidation resistance of the coated silicon carbide fiber. In some embodiments of the present invention, the preparation method may specifically include:

[0032] S1. Deposit a layer of rare earth modified lanthanum phosphate coating in situ on the surface of the silicon carbide fiber by hydrothermal method, and then dry it.

[0033] Specifically, in some embodiments, the in-situ deposition of a layer of rare earth modified lanthanum phosphate coating on the surface of the silicon carbide fiber by hydrothermal method includes: immersing the silicon carbide fiber in a layer containing La 3+ , rare earth ions and modifiers in phosphoric acid solution for hydrothermal treatment.

[0034] Among them, containing La 3+ The preparation step of the phosphoric acid solution of the rare earth ions and the modifying agent may include: mixing the solution obtained by mixing the lanthanum compound, the rare eart...

Embodiment 1

[0057] (1) Cook the SiC fibers with boiling water for more than 30 minutes, then place the SiC fibers in an oven at 120°C to dry for more than 30 minutes to remove the moisture on the surface of the fibers, then move the fibers into an atmosphere furnace with nitrogen as a protective gas to ensure that the oxygen partial pressure is not high. At a pressure higher than 0.05 standard atmosphere, treat at 1000°C for 2 hours, and then take out the SiC fiber after cooling with the furnace.

[0058] (2) La(NO 3 ) 3 ·6H 2 O, Ce(NO 3 ) 3 ·6H 2 O is configured into a solution of 100mL at a molar ratio of 9:1, where La 3+ The concentration is 1mol / L, add 5mL triethylenetetramine, mix well, put the solution in the refrigerator at 4℃ for more than 8h; 3 PO 4 Prepare 100 mL of a solution with a concentration of 1 mol / L, and place it in a refrigerator at 4°C for more than 8 hours. After mixing the above two solutions evenly, immerse the SiC fiber in the mixed solution, and move it i...

Embodiment 2

[0063] (1) Cook the SiC fiber with boiling water for more than 30 minutes, place the SiC fiber in an oven at 120°C to dry for more than 30 minutes to remove the moisture on the surface of the fiber, and then move the fiber into the atmosphere furnace with nitrogen as the protective gas to ensure that the oxygen partial pressure is At 0.01 standard atmospheric pressure, treat at 1000°C for 2 hours, and then take out the SiC fiber after cooling in the furnace.

[0064] (2) LaCl, YCl 3 According to the molar ratio of 19:1, it is configured into a solution of 100mL, in which La 3+ The concentration is 1mol / L, add 0.2g cetyltrimethylammonium bromide, mix well and put the solution in a refrigerator at 4°C for more than 8h; 3 PO 4 Prepare 100 mL of a solution with a concentration of 1 mol / L, and place it in a refrigerator at 4°C for more than 8 hours. After mixing the above two solutions evenly, immerse the SiC fiber in the mixed solution, and move it into the ultrasonic cleaning ...

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Abstract

The invention discloses a silicon carbide fiber material with a rare earth modified lanthanum phosphate coating, and a preparation method and application thereof. The preparation method of the siliconcarbide fiber material comprises the following steps: depositing the rare earth modified lanthanum phosphate coating on the surface of a silicon carbide fiber, and sintering the silicon carbide fiberdeposited with the rare earth modified lanthanum phosphate coating. The rare earth element in the rare earth modified lanthanum phosphate coating can reduce the reaction between LaPO4 and SiC in a high-temperature reducing atmosphere, so that the problem that the degradation performance of the existing silicon carbide fiber with the LaPO4 coating in the high-temperature reducing atmosphere is reduced is solved, the application of the LaPO4 coating in a non-oxidation ceramic matrix composite material system is expanded, and a ceramic-based composite material containing the silicon carbide fiber has a wide application prospect in the fields of aerospace and the like.

Description

technical field [0001] The invention relates to the technical field of inorganic non-metallic surface treatment, in particular to a silicon carbide fiber material with a rare earth modified lanthanum phosphate coating and a preparation method and application thereof. Background technique [0002] Silicon carbide (SiC) fibers have high strength, good fatigue resistance and creep resistance, excellent high temperature resistance, oxidation resistance and other characteristics, and are usually used as toughening resin matrix composites or ceramic matrix composites Mutually. In order to prevent the cracks in the composite material from directly cutting into and damaging the fibers, it is necessary to coat an interfacial functional coating between the matrix and the fibers to transmit loads and deflect cracks, thereby greatly improving the toughness of the material. [0003] Generally speaking, in the non-oxide ceramic matrix composite system, SiC fiber is the most common toughe...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): C04B41/87C04B35/80
CPCC04B41/87C04B41/5048C04B41/009C04B35/80C04B41/4529C04B41/0072C04B35/62281
Inventor 谭僖朱晖朝张小锋朱霞高张程陈焕涛邓春明
Owner GUANGDONG INST OF NEW MATERIALS