Benzothiadiazole Derivatives and Their Applications in Organic Electronic Devices
An organic electronic device, benzothiadiazole technology, applied in the field of solar energy, to achieve the effects of wide absorption range, high photoelectric conversion efficiency, and long device life
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Embodiment 1
[0109] Example 1: Synthesis of Compound 1
[0110]
[0111] Add 1-1 (5.13g, 5mmol), 1-2 (6.70g, 25mmol) and pyridine (5mL) to a 500mL two-necked flask, then pump argon three times, add 250mL of chloroform under argon protection, and at 65 °C to react for 24 hours. Cool to room temperature, extract three times with dichloromethane, combine the organic phases, dry and filter, add silica gel to spin dry, and separate and purify by column chromatography (n-hexane:dichloromethane=3:1) to obtain 3.05 g of white powder, yield 40% . MS(EI)m / z:[M]+:1027.69.
Embodiment 2
[0112] Example 2: Synthesis of Compound 2
[0113]
[0114] 2-1 (6.16 g, 6 mmol), 2-2 (11.85 g, 30 mmol) and pyridine (6 mL) were then pumped with argon three times, and 300 mL of chloroform was added under argon protection, and the reaction was carried out at 65° C. for 24 hours. Cool to room temperature, extract three times with dichloromethane, combine the organic phases, dry and filter, add silica gel to spin dry, and separate and purify by column chromatography (n-hexane:dichloromethane=3:1) to obtain 2.69 g of white powder, yield 38% . MS(EI)m / z:[M]+:1781.77.
Embodiment 3
[0115] Example 3: Synthesis of Compound 3
[0116]
[0117] 3-1 (5.13 g, 5 mmol), 3-2 (13.05 g, 25 mmol) and pyridine (6 mL) were then pumped with argon three times, and 300 mL of chloroform was added under argon protection, and the reaction was carried out at 65° C. for 24 hours. Cool to room temperature, extract three times with dichloromethane, combine the organic phases, dry and filter, add silica gel to spin dry, and separate and purify by column chromatography (n-hexane:dichloromethane=3:1) to obtain 3.76 g of white powder, yield 37% . MS(EI)m / z:[M]+:2035.86.
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