Polyamide-amine type branch-shape polymer nano materials, synthesis method and use thereof
A nanomaterial and dendritic technology, applied in the field of materials science, can solve the problems of difficulty in obtaining meaningful gene expression and low transduction efficiency
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Embodiment 1
[0018] Synthesis of G5 polyamide-amine dendrimers
[0019] 1. Pretreatment of raw materials
[0020] Methanol was added magnesium powder, refluxed for 4h and then purified by distillation. Add sodium hydroxide to ethylenediamine, let it stand for 24h, and purify by distillation. Methyl acrylate was added with anhydrous calcium chloride, refluxed for 4 hours and purified by distillation.
[0021] 2. Synthesis of G5 PAMAM dendrimer
[0022] Synthesis of generation 0.5 (G0.5): Take 0.7ml (10mmol) of ethylenediamine in a round bottom flask, add 20ml of methanol, slowly add 9.0ml (100mmol) of methyl acrylate dropwise, and stir electromagnetically at room temperature for 3d. After the reaction was completed, methanol and excess methyl acrylate were removed by rotary evaporation to obtain 3.8 g of light yellow viscous liquid. Yield 94.1%.
[0023] Synthesis of generation 1 (G1): Take 3.8 g of G0.5 obtained in the previous step, add 40 ml of methanol, slowly add 20 ml of ethylene...
Embodiment 2
[0025] Example 2 Gene transfection of hematopoietic stem cells
[0026] 1. Purification of Hematopoietic Stem Cells
[0027] The umbilical cord blood collected for no more than 4 hours was separated from mononuclear cells by Ficoll, and CD34-positive hematopoietic stem cells were separated by CD34 immunomagnetic beads, and the purity reached 95% by flow cytometry. Cultured for one day in serum-free medium containing hematopoietic stem cell growth factor.
[0028] 2. Gene Transfection of Hematopoietic Stem Cells
[0029] After the plasmid DNA containing the target gene is purified with an endotoxin-free plasmid extraction kit, it is diluted to 1 ug / ul with TE buffer, and the prepared nanoparticles are made into a 5 mg / ml aqueous solution, and the nanoparticles and plasmid DNA are mixed at a ratio of 5: 1, mixed evenly, added dropwise to the hematopoietic stem cell culture system, cultivated in a carbon dioxide incubator at 37°C for 2 hours, centrifuged and washed once, added ...
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