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Electrochemical preparation method of nano porous palladium

A nanoporous and electrochemical technology, applied in the field of electrochemical preparation of nanoporous palladium, can solve problems such as poor working conditions, toxicity and irritation, and serious environmental pollution, and achieve the effect of reducing production costs

Inactive Publication Date: 2011-11-23
UNIV OF JINAN
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0004] In addition, in the reported preparation methods, whether it is chemical corrosion or electrochemical dealloying, corrosive strong acid or strong alkali solution is used, the environmental pollution is relatively serious, toxic and irritating, and the working conditions are poor.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0022] (1) According to the ratio of 20% Pd by atomic percentage, and the rest is Al, put pure metal Al and Pd into a smelting furnace and heat to a molten state, and alloy them after sufficient stirring. Use argon to quickly blow out the molten liquid under a pressure of 0.1MPa, and chill it on a high-speed rotating copper roller with a cooling rate of 10 5 K / s, obtain a thin alloy strip with a thickness of 20-50 microns, a width of 2-5 mm, and a length of 1-10 cm;

[0023] (2) At 25°C, with the Al-Pd alloy as the working electrode, the platinum sheet as the counter electrode, the saturated calomel electrode as the reference electrode, and the 10wt% sodium chloride solution as the electrolyte, the overvoltage is 0.5V, and the electrochemical Dealloying treatment for 1 hour;

[0024] (3) Collect the reacted product, and rinse it repeatedly with distilled water until the electrolyte solution is completely washed (extensive pH test paper checks that the rinsed distilled water i...

Embodiment 2

[0026] (1) According to the ratio of 30% Pd by atomic percentage, and the rest is Al, put pure metal Al and Pd into a smelting furnace and heat them to a molten state, and alloy them after sufficient stirring. Use nitrogen to blow out the molten liquid rapidly under the pressure of 0.5MPa, and chill it on a high-speed rotating copper roller with a cooling rate of 10 3 K / s, obtain a thin alloy strip with a thickness of 20-40 microns, a width of 2-5 mm, and a length of 5-10 cm;

[0027] (2) At 60°C, with Al-Pd alloy as the working electrode, platinum wire as the counter electrode, a saturated silver chloride electrode as the reference electrode, 26wt% sodium chloride solution as the electrolyte, and an overvoltage of 1.0V, the electrode Chemical dealloying treatment for 0.5 hours;

[0028] (3) Collect the reacted product, and rinse it repeatedly with distilled water until the electrolyte solution is completely washed (extensive pH test paper checks that the rinsed distilled wat...

Embodiment 3

[0030] (1) According to the ratio of 40% Pd by atomic percentage, and the rest is Al, put pure metal Al and Pd into a smelting furnace and heat them to a molten state, and alloy them after sufficient stirring. The molten liquid is quickly blown out with nitrogen gas under a pressure of 1MPa, chilled on a high-speed rotating copper roller, and the cooling rate is 10 6 K / s, obtaining a thin alloy strip with a thickness of 20-40 microns, a width of 2-5 mm, and a length of 2-5 cm;

[0031] (2) Under 90 ℃, with Al-Pd alloy as working electrode, platinum plate as counter electrode, saturated silver chloride electrode as reference electrode, 25wt% potassium chloride solution as electrolyte, overvoltage is 1.0V, carry out electroplating Chemical dealloying treatment for 0.1 hour;

[0032] (3) Collect the reacted product, and rinse it repeatedly with distilled water until the electrolyte solution is completely washed (extensive pH test paper checks that the rinsed distilled water is n...

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Abstract

The invention discloses an electrochemical preparation method of nano porous palladium, comprising the following steps of: heating metallic aluminium and palladium in a smelter hearth to a molten state, and then sufficiently stirring so as to enable molten Al-Pd alloy to be alloyed; rapidly blowing off the molten Al-Pd alloy by utilizing inert gas and enabling the molten Al-Pd alloy to be rapidlysolidified on a copper roller rotating at high speed to form an Al-Pd alloy strip; carrying out electrochemical dealloying treatment on the prepared Al-Pd alloy strip in a neutral electrolyte solution; and washing the sample after being dealloyed in distilled water to be neutral, thereby preparing the nano porous palladium. The electrolyte solution adopted by the invention is a neutral solution without toxin or stimulation and is friendly to environment; the pore structure, the dimensions and the distribution of the nano porous palladium can be regulated and controlled according to the components, the working voltage, the working temperature and the dealloying time of the Al-Pd alloy.

Description

technical field [0001] The invention relates to an electrochemical preparation method of nanoporous palladium, which belongs to the technical field of preparation methods of nanometer materials. Background technique [0002] Nanoporous metals are materials with nanometer-sized pores ranging in size from a few nanometers to hundreds of nanometers. Nanoporous metals have a unique pore structure, nanoscale pore size and high specific surface area, and exhibit unique physical, chemical and mechanical properties, so they have great application potential in many fields, such as fuel cells, sensing, excitation , gas-phase and liquid-phase catalysis, surface-enhanced Raman scattering, microfluidic control, etc. At present, platinum-based catalysts are most widely used in the field of fuel cells, but they are easily poisoned and expensive. Compared with platinum, the price of palladium is one-fourth to one-fifth, and it has higher catalytic activity. Meanwhile, palladium is an imp...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C25C5/02
Inventor 王艳张忠华
Owner UNIV OF JINAN