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Nanofiber membrane fabric with self-cleaning carbon nanotube modification and preparation method

A technology of carbon nanotube modification and nanofiber membrane, which is applied in fiber treatment, chemical instruments and methods, non-woven fabrics, etc., can solve the problems of composite material performance impact, low air permeability, high production cost, etc. Enhanced self-cleaning performance, excellent air permeability, and easy-to-obtain raw materials

Active Publication Date: 2016-08-24
符思敏
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0004] However, on the one hand, due to its high specific surface area, carbon nanotubes are easy to form aggregate structures in solvents or polymer matrices, which will affect the performance of composite materials; on the other hand, introducing carbon nanotubes into polymers In the process of polymer modification, there are often cumbersome processes and low air permeability (usually at 0.05cm 3 / cm 2 / s), high production costs, serious environmental pollution and other disadvantages

Method used

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Examples

Experimental program
Comparison scheme
Effect test

preparation example Construction

[0019] The steps of the preparation method of the electrospun nanofiber membrane fabric with self-cleaning carbon nanotube modification are as follows:

[0020] 1) Weigh a certain amount of multi-walled carbon nanotubes and disperse them in 60 mL of 4.0 mol / L HCl. After ultrasonic treatment for 2-3 h, wash with twice distilled water until neutral. 60 mL HNO 3 + H 2 SO 4 (Volume ratio 1:3) Ultrasonic treatment for 4-5 h, washed with deionized water until the pH is neutral, placed in a vacuum oven at 60-80°C for 6-10 h, and obtained surface modification by acid treatment and functionalization. Sexual carbon nanotubes;

[0021] 2) Dry the polymer at 60-90°C for 0.5-2 hours, then add it to the solvent, and stir evenly for 4-6 hours under airtight conditions at 80°C to fully dissolve it, and the solution is colorless Transparent liquid, to obtain a high molecular polymer solution with a concentration of 15% to 25%;

[0022] 3) A certain amount of carbon nanotubes is added to ...

Embodiment 1

[0027] 1) Weigh 1 g of multi-walled carbon nanotubes and disperse them in 60 mL of 4.0 mol / L HCl. After ultrasonic treatment for 2 hours, wash with twice distilled water until neutral. 60 mL HNO 3 + H 2 SO 4 (Volume ratio 1:3) Sonicate for 4 h, wash with deionized water until the pH is neutral, place in a vacuum oven at 60°C for 10 h in vacuum, and obtain surface-modified carbon nanotubes by acid treatment and functionalization;

[0028] 2) Dry 10g of PU at 60°C for 2 hours, then add it to 55g of N,N-dimethylformamide, and stir evenly at 80°C for 4 hours under airtight conditions to fully dissolve it, and the solution is free Color transparent liquid, obtains the PU solution that concentration is 15%;

[0029] 3) Add 0.075g of carbon nanotubes to 10g of N,N-dimethylformamide, and ultrasonically treat for 2 hours at room temperature to obtain a uniformly dispersed modified carbon nanotube solution;

[0030] 4) Add the dispersed carbon nanotube solution into the PU solution...

Embodiment 2

[0033] 1) Weigh 2 g of multi-walled carbon nanotubes and disperse them in 60 mL of 4.0 mol / L HCl. After ultrasonic treatment for 3 h, wash with twice distilled water until neutral. 60 mL HNO 3 + H 2 SO 4 (Volume ratio 1:3) Sonicate for 5 h, wash with deionized water until the pH is neutral, place in a vacuum oven at 80°C for 10 h in vacuum, and obtain surface-modified carbon nanotubes by acid treatment and functionalization;

[0034] 2) Dry 10g of PMMA at 90°C for 0.5 h, then add it to 55g of N,N-dimethylacetamide, stir evenly at 80°C for 4 h to fully dissolve, and the solution is colorless and transparent Liquid, obtaining concentration is the PMMA solution of 15%;

[0035] 3) Add 0.075g of carbon nanotubes to 10g of N,N-dimethylacetamide, and ultrasonically treat for 2 hours at room temperature to obtain a uniformly dispersed modified carbon nanotube solution;

[0036]4) Add the dispersed carbon nanotube solution into the PMMA solution and blend for 4 hours to obtain a ...

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PUM

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Abstract

The invention discloses a self-cleaning carbon nanotube modified electrostatic spinning nanofiber membrane fabric and a preparation method. Self-cleaning nanofiber membrane fabric modified by carbon nanotubes, carbon nanotube-modified polymer coated on the structural fiber fabric, the diameter of the nanofibers is 150-500nm, and the film thickness is 0.02mm , through the carbon nanotubes all over the surface of the membrane, the hydrophobicity and self-cleaning of the nanofiber membrane fabric are enhanced, the air permeability is between 0.4-0.6 cm3 / cm2 / s, and the waterproof performance is between 35-40 cm H2O . The polymer nanofiber membrane fabric obtained in the present invention not only has excellent air permeability, but also has good waterproof performance. It has great application and industrialization value.

Description

technical field [0001] The invention relates to the field of special nanofiber materials, in particular to a preparation method of a self-cleaning carbon nanotube modified nanofiber membrane fabric. Background technique [0002] Due to the unique flexibility, wear resistance, bacteria resistance and solvent resistance of high molecular polymer, it is widely used in the coating of medium and high-grade fabrics. With the development of film fabrics, polymer fabrics with waterproof and breathable properties prepared by solvent / non-solvent technology, dry coating technology, high boiling point organic droplet technology and melt extrusion molding are used in environmental protection materials, High-grade clothing and medical textiles have been widely used. [0003] Carbon nanotubes are coaxial circular tubes with several to tens of layers of carbon atoms arranged in a hexagonal shape, with a diameter ranging from a few nanometers to tens of nanometers. Since carbon nanotubes w...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B32B27/02D04H1/728D01D5/00
Inventor 符思敏费辉周建伟刘创
Owner 符思敏