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Method for preparing tripolyglycerol fatty acid ester by solid superacid catalysis

A technology of triglyceride and solid superacid, which is applied in chemical instruments and methods, fatty acid esterification, fatty acid chemical modification, etc., can solve the problems of low esterification rate and low product purity, and achieve low corrosion and high purity High, high yield effect

Active Publication Date: 2015-04-22
GUANGZHOU CARDLO BIOCHEM TECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

However, this method still needs to consider issues such as catalyst cost, catalytic efficiency and the development of new reactors.
At the same time, there are technical problems that the esterification rate is low and the purity of the product obtained is low, which has brought great restrictions for wide application.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0030] Solid Superacid SO 4 2- / ZrO 2 -SiO 2 preparation of

[0031] The specific steps are: take zirconium oxychloride (ZrOCl 2 ·8H 2 O) Prepare 100g of 3% zirconium oxychloride solution, add 33.3g of diatomaceous earth, and let it stand for about 20 minutes to fully impregnate it. Then 25% concentrated ammonia water was added to adjust the pH to 8.5, and after standing for 4 hours, it was suction filtered and washed with distilled water for 3 times, and the obtained precipitate was dried in an oven at 80°C for 1 hour. After drying, 30 g was added to 300 g of 50 wt% sulfuric acid solution for immersion for 20 min, and then suction filtered again. Finally, the filter cake was dried in an oven at 80 °C for 0.5 h, and then transferred to a muffle furnace at 600 °C for 3 h to obtain SO 4 2- / ZrO 2 -SiO 2 Solid superacid catalyst.

[0032] Preparation of triglyceride: heat 10kg glycerin and 9g strong acidic cation exchange resin (D001SS macroporous strong acidic styrene...

Embodiment 2

[0035] Solid Superacid SO 4 2- / ZrO 2 -SiO 2 preparation of

[0036] The specific steps are: take zirconium oxychloride (ZrOCl 2 ·8H 2 O) Prepare 100g of 4% zirconium oxychloride solution, add 40g of diatomaceous earth, and let it stand for about 20 minutes to fully impregnate it. Then 28% concentrated ammonia water was added to adjust the pH to 9, and after standing for 5 h, it was suction filtered and washed with distilled water three times, and the obtained precipitate was dried in an oven at 80 °C for 1 h. After drying, 40 g was added to 800 g of 50 wt% sulfuric acid solution for immersion for 20 min, and then suction filtered again. Finally, the filter cake was dried in an oven at 80 °C for 0.5 h, and then transferred to a muffle furnace at 600 °C for 3 h to obtain SO 4 2- / ZrO 2 -SiO 2 Solid superacid catalyst.

[0037] Preparation of triglycerides: Heat 10kg of glycerin and 9g of strongly acidic cation exchange resin (D001SS macroporous strongly acidic styren...

Embodiment 3

[0040] Solid Superacid SO 4 2- / ZrO 2 -SiO 2 preparation of

[0041] The specific steps are: take zirconium oxychloride (ZrOCl 2 ·8H 2 O) Prepare 100g of 5% zirconium oxychloride solution, add 60g of diatomaceous earth, and let it stand for about 20 minutes to fully impregnate it. Then 28% concentrated ammonia water was added to adjust the pH to 8, and after standing for 5 h, it was suction filtered and washed with distilled water for 3 times, and the obtained precipitate was dried in an oven at 80 °C for 1 h. After drying, 60 g was added to 300 g of 50 wt% sulfuric acid solution for immersion for 20 min, and then suction filtered again. Finally, the filter cake was dried in an oven at 80 °C for 0.5 h, and then transferred to a muffle furnace at 600 °C for 3 h to obtain SO 4 2- / ZrO 2 -SiO 2 Solid superacid catalyst.

[0042] Preparation of triglycerides: Heat 10kg of glycerin and 9g of strongly acidic cation exchange resin (D001SS macroporous strongly acidic styren...

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Abstract

The invention relates to a method for preparing tripolyglycerol fatty acid ester by solid superacid catalysis. The method comprises the following steps that triglycerol is prepared and the triglycerol and aliphatic acid undergoes a reaction in the presence of solid superacid. The method realizes tripolyglycerol fatty acid ester synthesis by a heterogeneous-phase high-viscosity reaction system. The method utilizes the raw materials which can be separated easily and can be recycled so that a cost is reduced. The method has a high tripolyglycerol fatty acid ester yield and has an esterification rate more than 97%. The prepared tripolyglycerol fatty acid ester has high purity and has free fatty acid content less than 0.1%.

Description

technical field [0001] The invention belongs to the field of chemical synthesis, and in particular relates to a method for preparing triglycerides by solid superacid catalysis. Background technique [0002] Polyglycerol fatty acid ester (referred to as polyglycerol ester, PGFE) is an ester formed of polyglycerol and fatty acid, and its structure varies according to the degree of polymerization of glycerin, the type of fatty acid and the degree of esterification. Polyglycerol ester is a polyhydroxy ester nonionic surfactant. Because its hydrophilicity increases with the increase of the degree of polymerization of glycerin lipids, and the lipophilicity varies with the difference of fatty acid lipids, so by changing the degree of polymerization of glycerin, the Depending on the type and degree of esterification, surfactants with different properties can be obtained with HLB values ​​ranging from 1 to 16. The interval can be adjusted arbitrarily, so it can be used as O / W emulsi...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): C11C3/02B01J27/053
CPCB01J27/053C11C3/02C11C3/025
Inventor 徐怀义
Owner GUANGZHOU CARDLO BIOCHEM TECH