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A preparation method of fluorine-containing copolymer for water treatment membrane

A technology for water treatment membranes and copolymers, applied in the field of preparation of fluorine-containing copolymers, can solve the problems of poor chemical corrosion resistance and weather resistance, difficult to obtain structural copolymers, poor chemical stability, etc., so as to maintain chemical stability. and weather resistance, high product purity, good hydrophilic effect

Active Publication Date: 2017-01-11
RUYUAN DONGYANG LIGHT FLUORINE RESIN CO LTD
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

However, there are two problems with the use of acrylic acid monomers. One is that diol monoacrylate is a monomer with a very fast polymerization rate. It is easy to self-polymerize when it is copolymerized with fluorine-containing monomers, and it is not easy to obtain a copolymer with a regular structure; The second is that the chemical stability of the monoacrylate glycol ester unit in the copolymer is poor, and it is easy to degrade, and its chemical corrosion resistance and weather resistance are far inferior to those of polyvinylidene fluoride

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0031] In a cleaned 5 L vertical autoclave, 2.6 L of deionized water containing a mixture of 5.2 g of methylcellulose and hydroxyethylcellulose (1:1) was added. Vacuumize and replace nitrogen 5 times until the oxygen content is lower than 30ppm. Add 5.0 g of acetone into the reaction kettle, adjust the stirring speed to 200 r / min, and maintain the temperature at 15°C. Vinylidene fluoride and hexafluoropropylene were added to the reaction kettle at a molar ratio of 90:5, and the temperature was raised to 40°C. When the pressure in the kettle reached 4.0MPa, 6.0g of diisopropyl peroxydicarbonate and 35 g of 2-trifluoromethacrylic acid in water. Subsequently, the temperature of the reactor was raised to 60° C. at a rate of 10° C. / h, and the stirring speed was increased to 600 r / min. During the polymerization process, the ratio of additional monomer vinylidene fluoride, hexafluoropropylene and 2-trifluoromethacrylic acid is 90:5:5, so that the reaction pressure is maintained at ...

Embodiment 2

[0042] In a cleaned 5 L vertical autoclave, 2.6 L of deionized water containing a mixture of 6.0 g of methylcellulose and hydroxyethylcellulose (1:1) was added. Vacuumize and replace nitrogen 5 times until the oxygen content is lower than 30ppm. Add 6.0 g of acetone into the reaction kettle, adjust the stirring speed to 200 r / min, and maintain the temperature at 20°C. Vinylidene fluoride and hexafluoropropylene were added to the reaction kettle at a molar ratio of 75:20, the temperature was raised to 40°C, and when the pressure in the kettle reached 4.0MPa, 6.0g of diisopropyl peroxydicarbonate and 35 g of 2-trifluoromethacrylic acid in water. Subsequently, the temperature of the reactor was raised to 70° C. at a rate of 15° C. / h, while the stirring speed was increased to 600 r / min. During the polymerization process, monomers with a ratio of vinylidene fluoride / hexafluoropropylene / 2-trifluoromethacrylic acid of 75:20:5 were added to maintain the reaction pressure at 4.8MPa. ...

Embodiment 3

[0044] In a cleaned 5L vertical autoclave, 2.6L of deionized water containing a mixture of 5.5g of methylcellulose and hydroxyethylcellulose (1:1) was added. Vacuumize and replace nitrogen 5 times until the oxygen content is lower than 30ppm. Add 5.5 g of acetone into the reactor, adjust the stirring speed to 200 r / min, and maintain the temperature at 15°C. Vinylidene fluoride and hexafluoropropylene were added to the reaction kettle at a molar ratio of 80:10, and the temperature was raised to 40°C. When the pressure in the kettle reached 4.0MPa, 6.0g of diisopropyl peroxydicarbonate and 70 g of 2-trifluoromethacrylic acid in water. Subsequently, the temperature of the reactor was raised to 70° C. at a rate of 15° C. / h, while the stirring speed was increased to 600 r / min. During the polymerization process, add monomers with a ratio of vinylidene fluoride / hexafluoropropylene / 2-trifluoromethacrylic acid of 80:10:10 to maintain the reaction pressure at 5.5 MPa, and finish the r...

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Abstract

The invention relates to a method for preparing fluorine-containing copolymer used for a water treatment film. According to the method, three kinds of monomer including VDF (vinylidene difluoride), HFP (hexafluoropropylene) and 2-trifluoromethyl acrylic acid are subjected to copolymerization. The method comprises steps as follows: mixed monomer of a chain transfer agent, VDF and HFP is added to a reaction kettle containing a dispersing agent aqueous solution and uniformly mixed, then an aqueous solution of an initiating agent and 2-trifluoromethyl acrylic acid monomer is added, and after a reaction is performed for 3-8h, a terpolymer suspension liquid is filtered, washed, dried and smashed to obtain a powdery product. The prepared polyvinylidene fluoride suspension liquid is filtered, washed and dried and then the powdery product is obtained. The thermal stability and the physical and mechanical performance of the fluorine-containing copolymer powder are good, the reaction process is simple, and the method is suitable for industrial production.

Description

technical field [0001] The invention relates to the field of preparation of fluorine-containing copolymers, in particular to a preparation method of a fluorine-containing copolymer that can be used for water treatment membranes. Background technique [0002] The binary copolymer of vinylidene fluoride (VDF) and hexafluoropropylene (HFP) is a fluorine-containing copolymer with excellent performance. This copolymer has excellent thermal stability, chemical resistance and abrasion resistance. It is A self-extinguishing material resistant to UV degradation. Compared with polyvinylidene fluoride, vinylidene fluoride copolymer containing a small amount of hexafluoropropylene has better toughness, is not easy to crack, and has better strength. It has become an ideal raw material for the production of water treatment membranes. However, due to the low surface energy of this copolymer and the inability to form hydrogen bonds with water molecules, it has extremely strong hydrophobici...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C08F214/22C08F214/28C08F220/04C08F2/38C08F2/20C08F4/36B01D71/32
Inventor 姚文强汤诚王寅飞
Owner RUYUAN DONGYANG LIGHT FLUORINE RESIN CO LTD