A kind of calcium phosphate nanoparticles embedding cisplatin and its preparation method and application
A nanoparticle and calcium phosphate technology, which is applied in the field of preparation of calcium phosphate nanoparticles, can solve the problem of reducing the killing effect of tumor cells, and achieve the effects of controllable synthesis method, good biocompatibility, and mild preparation conditions
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Embodiment 1
[0055] Embodiment 1, the synthesis and characterization of hydrophilic block copolymer PEG-PAA
[0056] 1. Synthesis of hydrophilic copolymer PEG-PAA
[0057] The hydrophilic block copolymer PEG-PAA is made of ETP-PEG 5K It is obtained by polymerization under the catalytic conditions of AIBN.
[0058] 1. Synthesis of reversible addition-fragmentation chain transfer polymerization reagent (ETP)
[0059] The synthetic route of reversible addition-fragmentation chain transfer polymerization reagent (ETP) is as follows figure 1 Shown: ethanethiol (24.852g, 400mmol) and 60mL of distilled water are mixed and stirred, then slowly dropwise add 32g of a mass concentration of 50% NaOH solution (wherein NaOH 16g, 400mmol) in an ice bath, and then Add 20mL of acetone under the condition and stir for 30min. Then carbon disulfide (34.2 g, 450 mmol) was added and the solution turned into a clear orange, and stirred for 30 min. 2-Bromopropionic acid (62.73 g, 410 mmol) was slowly added d...
Embodiment 2
[0074] Example 2, Preparation and Characterization of Calcium Phosphate Nanoparticles Encapsulating Cisplatin
[0075] 1. Preparation of cisplatin-encapsulated calcium phosphate nanoparticles (CaP NP / CDDP)
[0076] Amphiphilic block copolymers have been extensively studied as drug delivery vehicles. When amphiphilic block copolymers are dissolved in a good solvent for one block and a poor solvent for the other block, the copolymers spontaneously assemble into aggregates.
[0077] However, the method of forming micelles with hydrophilic block copolymers is rarely used. In this description, part of the carboxyl group of the hydrophilic block copolymer PEG-PAA is coordinated with cisplatin to connect the cisplatin to the copolymer, and then use the method of calcium ion micelle nucleation to make the hydrophilic block copolymer Micelles are formed, and finally the micelles are combined with hydrogen phosphate to form a calcium phosphate mineral layer, so that cisplatin can be e...
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