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A kind of chitin nanocrystal composite polysulfone hollow fiber membrane and preparation method thereof

A technology of chitin nanocrystals and fiber membranes, applied in the field of separation membranes, can solve the problems of industrial production limitations, poor membrane surface quality, and difficulty in membrane production, and achieve the effect of improving mechanical strength, improving comprehensive performance, and simple and easy methods

Active Publication Date: 2019-07-05
QINYUAN GRP CO LTD
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Polyethylene glycol and polyvinylpyrrolidone with high molecular weight or high content can increase the viscosity of the casting solution system and obtain a polysulfone membrane with a sponge pore structure, but there are also shortcomings such as poor membrane surface quality, low strength, and difficulty in membrane production, making it Industrial production is limited

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0033] Chitin nanocrystals with a diameter of 4 nm and a length of 40 nm were uniformly dispersed in dimethylacetamide, polysulfone and sulfonated polysulfone with a sulfonation degree of 20% were added, stirred and dissolved into a uniform solution, and allowed to stand Degassing to obtain the casting solution, the formula of the casting solution by mass percentage is: polysulfone 12%, chitin nanocrystal 0.2%, sulfonated polysulfone 1.5%, dimethylacetamide 86.3%; dimethylacetamide A mixed solution of amide and water with a volume ratio of 1:3 was used as the core fluid. The casting liquid and the core liquid are simultaneously extruded through the annular spinning head of the submerged precipitation phase inversion spinning device to form a tubular liquid film. The flow rate of the casting liquid is 20 g / min, the flow rate of the core liquid is 20 ml / min, and the tubular liquid film After passing through an air gap of 7 cm, enter the coagulation bath of water and solidify for...

Embodiment 2

[0036] Chitin nanocrystals with a diameter of 10 nm and a length of 300 nm were uniformly dispersed in dimethyl sulfoxide, polysulfone and sulfonated polysulfone with a sulfonation degree of 50% were added, stirred and dissolved into a uniform solution, and allowed to stand Degassing to obtain the casting solution, the formulation of the casting solution by mass percentage is: polysulfone 20%, chitin nanocrystal 2%, sulfonated polysulfone 7%, dimethyl sulfoxide 71%; dimethyl sulfoxide A mixed solution of sulfone and water with a volume ratio of 1:4 was used as the core fluid. The casting liquid and the core liquid were simultaneously extruded through the annular spinning head of the submerged precipitation phase inversion spinning device to form a tubular liquid film. The flow rate of the casting liquid was 10 g / min, and the flow rate of the core liquid was 10 ml / min. After passing through an air gap of 15 cm, the membrane was solidified in a water coagulation bath for 24 hour...

Embodiment 3

[0039]Chitin nanocrystals with a diameter of 10 nm and a length of 100 nm were uniformly dispersed in an organic solvent (a mixture of dimethylacetamide and dimethyl sulfoxide at a volume ratio of 1:1), and polysulfone and sulfone The sulfonated polysulfone with a sulfonation degree of 30% is stirred and dissolved into a uniform solution, left to stand for degassing, and a casting solution is obtained. The formula of the casting solution in terms of mass percentage is: 30% polysulfone, 4% chitin nanocrystals, Sulfonated polysulfone 3%, organic solvent 63%; the mixture of dimethylacetamide and dimethyl sulfoxide (dimethylacetamide and dimethyl sulfoxide mixed at a volume ratio of 1:1) and The water volume ratio is 1:3 mixed as the core fluid. The casting liquid and the core liquid are simultaneously extruded through the annular spinning head of the submerged precipitation phase inversion spinning device to form a tubular liquid film. The flow rate of the casting liquid is 10 g / ...

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Abstract

The invention discloses a chitin nanocrystalline-polysulfone composite hollow fiber membrane and a preparation method thereof. The chitin nanocrystalline-polysulfone composite hollow fiber membrane is obtained through the steps that a casting solution and a core solution are co-extruded by an annular spinning nozzle to form a tubular liquid membrane by adopting an immerse precipitation phase inversion method, and then the tubular liquid membrane is coagulated through a coagulating bath, wherein the casting solution is prepared by mixing, by mass, 12%-30% of polysulfone, 0.1%-7% of chitin nanocrystallines, 0.5%-7% of sulfonated polysulfone and the balance organic solvents. The chitin nanocrystalline-polysulfone composite hollow fiber membrane prepared through the method has the high strength and the good hydrophilicity and antibacterial property.

Description

technical field [0001] The invention relates to the technical field of separation membranes, in particular to a chitin nanocrystal composite polysulfone hollow fiber membrane and a preparation method thereof. Background technique [0002] Polysulfone membrane has excellent thermal stability and chemical stability, and is widely used in fields such as hemodialysis, seawater desalination and water treatment. The composition of the casting solution system and the film-forming conditions are important factors that determine the structure and performance of the polysulfone membrane. Therefore, by adjusting the concentration and composition of the casting solution, the composition of the coagulation bath, the temperature, the air gap and the flow rate, etc., different physical structures can be prepared. and performance polysulfone membranes. However, polysulfone is a highly hydrophobic polymer material. Therefore, the hydrophilicity of the polysulfone membrane is poor. When the ...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B01D69/08B01D69/02B01D67/00B01D71/68
CPCB01D67/0002B01D69/02B01D69/08B01D71/68B01D2325/24B01D2325/36B01D2325/48
Inventor 胡梦欣叶建荣沈立强
Owner QINYUAN GRP CO LTD