Catalytic nanoparticle-containing microporous chitosan particles and application thereof
A nano-catalysis, chitosan technology, applied in the separation of dispersed particles, physical/chemical process catalysts, organic compounds/hydrides/coordination complex catalysts, etc., can solve the problem of unfavorable recycling, low treatment concentration, secondary pollution and other problems, to achieve the effect of effective adsorption, uniform distribution and strong adsorption performance
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Embodiment 1
[0025] Example 1 Preparation of mesoporous chitosan particles containing nano-catalyst particles
[0026] Sample 1: Dissolve chitosan (deacetylation degree is above 80%, molecular weight is 5000-200,000) with 2% acetic acid into 0.5-5% chitosan solution, after the belt dissolves completely, put a certain amount of titanium Acetate methyl ester (the amount is 30% of chitosan mass) is added, stirs rapidly, after the reaction is complete, it becomes a gel, and the gel is freeze-dried to obtain nano-TiO 2 Mesoporous Chitosan Particles for Catalytic Particles, TiO 2 The particle size is 10-50nm.
[0027] Sample 2: Dissolve chitosan (deacetylation degree is above 80%, molecular weight is 5000-200,000) with 2% acetic acid into 0.5-5% chitosan solution, after the belt dissolves completely, add a certain amount of silicon Acetate methyl ester, (consumption is 30% of chitosan quality) adds, stirs rapidly, becomes gel after treating that reaction is complete, and gel is carried out fre...
Embodiment 2
[0029] Embodiment 2 formaldehyde adsorption experiment
[0030] Refer to "Diatomite-based Nano-TiO 2 Experimental Research on Formaldehyde Degradation" (Yu Chenglin, Quan Hongen, Kang Yong. [J]. Journal of Environmental Science, 2012, 32(1): 116-122), at room temperature, press 50g / m 2 The amount of the sample evenly distributed on the glass surface, under natural light, to measure the concentration of different formaldehyde (2mg / m 3 、6mg / m 3 , 10mg / m 3 ) The scavenging effect of the mesoporous chitosan particles containing nano catalytic particles of the present invention on formaldehyde gas. The results are shown in Table 1-3.
[0031] Table 1
[0032]
[0033] Table 2
[0034]
[0035] table 3
[0036]
[0037] The results show that the mesoporous chitosan particles containing nano catalytic particles of the present invention have a good scavenging effect on formaldehyde gas, wherein, 2mg / m 3 About 90% of formaldehyde, 10mg / m 3 Under ultra-high concentrati...
Embodiment 3
[0039] Using the method of dynamic gas distribution, the concentration of H 2 The mixture of S and nitrogen, and a small amount of air are mixed evenly in the mixer, and then enter the closed adsorption box bed unit at a flow rate of 0.3L / min, and the air is filled with CaCl before entering the mixer. 2 Dry the tubes to remove moisture from the air. At room temperature, according to 50g / m 2 The amount of the sample is evenly distributed on the glass surface, under natural light, measure the mesoporous chitosan particles containing nano catalytic particles of the present invention to 100mg / m 3 The scavenging effect of hydrogen sulfide gas under the concentration. The results are shown in Table 4. The results show that the mesoporous chitosan particles containing nano catalytic particles of the present invention have a good scavenging effect on hydrogen sulfide gas, and can reduce the concentration of hydrogen sulfide by more than 50% within 10 minutes. More than 99% clearan...
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Abstract
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