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Method for preparing oil-filled chlorinated polyethylene rubber by suspension chlorination reaction

A technology of chlorinated polyethylene and chlorination reaction, which is applied in the field of chlorinated polyethylene rubber preparation, can solve the problems of high content of chlorinated paraffin, high content of polyethylene wax, poor heat aging resistance, etc. The effect of high product performance and improved heat aging resistance

Inactive Publication Date: 2018-12-07
潍坊硕邑化学有限公司
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0004] The CM products currently on the market, in order to ensure their basic processing fluidity, all use high-density polyethylene with a wide molecular weight distribution as raw materials. The Mooney viscosity of the product is relatively low, and the mechanical strength of the product is also low.
In addition, the wide molecular weight distribution makes the content of polyethylene wax in CM products high, and the chlorinated polyethylene wax formed after being chlorinated enters the product to make the content of chlorinated paraffins high, resulting in poor heat aging resistance and not environmentally friendly

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0031] This embodiment provides a method for preparing oil-extended chlorinated polyethylene rubber by suspension chlorination reaction, the steps are as follows:

[0032] (1) Put 140Kg of 17% hydrochloric acid in a 200L glass-lined reactor, start stirring, select metallocene high-density polyethylene powder 40.0Kg, melt index MI (190℃ / 10min, 5Kg) 1, melt flow ratio MFR 9.5, poly Ethylene wax content 0.1%, water content 0.15wt%, particle size 90μm; hydrophobic white carbon black 0.06Kg, organic fluorine non-ionic surfactant 0.5Kg, benzoyl peroxide 0.04Kg, add to the reactor together, well mixed;

[0033] (2) Turn on the stirring, and heat the system to 75°C, pump the negative pressure to -0.08Mpa, feed chlorine gas, control the chlorine flow rate at 0.2-0.3Kg / min, when 25Kg chlorine gas is fed, the temperature of the material rises to 132.5°C , put cooling water into the jacket of the reaction kettle to cool down, and keep the material temperature at 132.5°C. When the total c...

Embodiment 2

[0041] This embodiment provides a method for preparing oil-extended chlorinated polyethylene rubber by suspension chlorination reaction, the steps are as follows:

[0042](1) Add 16000Kg 18% hydrochloric acid into a 25m³ glass-lined reactor, start stirring, select metallocene high-density polyethylene powder 2200Kg, melt index (MI 190°C / 10min, 5Kg) 4, melt flow ratio (MFR) 9.5, Water content 0.2wt%, particle size 150μm; hydrophobic white carbon black 8.8Kg, surfactant 40Kg, benzoyl peroxide 8.8Kg, add to the reactor together, mix well;

[0043] (2) Raise the temperature of the material to 76°C, pump negative pressure to make the pressure of the reactor -0.04Mpa, feed chlorine gas, control the speed of chlorine gas to make the pressure and temperature in the reactor rise slowly, when the mass number of chlorine gas introduced reaches 1330Kg, feed Cooling water was introduced into the jacket of the reaction kettle to transfer the excess heat of reaction, so that the reaction tem...

Embodiment 3

[0052] This embodiment provides a method for preparing oil-extended chlorinated polyethylene rubber by suspension chlorination reaction, the steps are as follows:

[0053] (1) Add 16000Kg 18% hydrochloric acid into a 25m³ glass-lined reactor, start stirring, select metallocene high-density polyethylene powder 2200Kg, melt index (MI 190°C / 10min, 5Kg) 2, melt flow ratio (MFR) 9.5, Water content 0.2wt%, particle size 120μm; hydrophobic white carbon black 8.8Kg, surfactant 40Kg, benzoyl peroxide 8.8Kg, add to the reactor together, mix well;

[0054] (2) Raise the temperature of the material to 76°C, pump negative pressure to make the pressure of the reactor -0.04Mpa, feed chlorine gas, control the speed of chlorine gas to make the pressure and temperature in the reactor rise slowly, when the mass number of chlorine gas introduced reaches 1330Kg, feed Cooling water was introduced into the jacket of the reaction kettle to transfer the excess heat of reaction, so that the reaction te...

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Abstract

The invention provides a method for preparing oil-filled chlorinated polyethylene rubber by a suspension chlorination reaction and belongs to the field of preparation of chlorinated polyethylene. Themethod comprises: putting hydrochloric acid in a glass-lined reactor, stirring the hydrochloric acid, adding high-density polyethylene powder, an anti-adhesive, a surfactant and an initiator into themixture, carrying out vacuum-pumping on the reactor, feeding chlorine into the reactor for a reaction to obtain a high Mooney viscosity chlorinated polyethylene-hydrochloric acid suspension liquid, putting the chlorinated polyethylene-hydrochloric acid suspension liquid into a vacuum rubber filter, dehydrating the materials through vacuum suction filtration, drying the materials through hot air toobtain high Mooney viscosity CM powder, putting the high Mooney viscosity chlorinated polyethylene rubber powder and rubber operating oil into a high-speed mixer and carrying out stirring to obtain oil-filled chlorinated polyethylene rubber particles or pieces. The oil-filled chlorinated polyethylene rubber has good heat aging resistance and high product rigidity. The method effectively reduces the production cost of the product. The production cost of the oil-filled CM is lower than that of the suspension method CM, and the mechanical performance is improved.

Description

technical field [0001] The invention belongs to the field of preparation of chlorinated polyethylene rubber, and in particular relates to a method for preparing oil-extended chlorinated polyethylene rubber by suspension chlorination reaction. Background technique [0002] Chlorinated polyethylene rubber (hereinafter referred to as CM) is a special synthetic rubber obtained from high-density polyethylene (hereinafter referred to as HDPE) through chlorination. Due to the saturation of the structure, the vulcanizate has excellent weather resistance, ozone resistance, oil resistance, chemical resistance, abrasion resistance, radiation resistance, flame retardancy and air tightness, and good color stability, so it is widely used Used in automotive rubber parts, flame retardant wires and cables, roof waterproofing and rubber dams, chemical equipment anti-corrosion linings, shoemaking and other fields. [0003] The production methods of chlorinated polyethylene rubber include solv...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): C08L23/28C08L91/00C08K3/36C08K5/098C08K13/02C08K5/12C08K5/11C08F8/22C08F110/02
CPCC08F8/22C08K3/36C08K5/098C08K5/11C08K5/12C08K13/02C08L23/286C08L2201/08C08F110/02C08L91/00
Inventor 李垂祥白杰孙振宇徐建华栾京民
Owner 潍坊硕邑化学有限公司