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Polylactic acid fiber reinforced polylactic acid/hydroxyapatite composite material and preparation method thereof

A technology of polylactic acid fiber and hydroxyapatite, which is applied in the direction of fiber chemical characteristics, rayon manufacturing, single-component polyester rayon, etc., can solve the problem of insufficient toughness of polylactic acid materials, and achieve safe impact resistance. Poisonous, strengthening toughness, strengthening the effect of antibacterial performance

Inactive Publication Date: 2019-01-22
林毅平
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0003] However, the toughness of polylactic acid material is not enough, so it is necessary to further improve the toughness of the material to further expand the application range of the material

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0021] A preparation method of polylactic acid / hydroxyapatite composite material reinforced by polylactic acid fiber, is characterized in that, comprises the following steps:

[0022] (1) Dried Scutellaria baicalensis and honeysuckle were crushed through a 60-mesh sieve, and the two kinds of Chinese medicine powders were mixed according to a mass ratio of 1:1. : After mixing at a mass volume ratio (g / mL) of 15, reflux extraction at 65°C for 3 hours and then filter, pass the filtrate through an ultrafiltration membrane with a molecular weight cut-off of 8000, spin dry, crush and sieve to obtain a natural antibacterial agent;

[0023] (2) Mix 12 parts of polylactic acid, 0.15 parts of natural antibacterial agent, 0.05 parts of gallic acid, 40 parts of N,N-dimethylformamide, and 47.8 parts of ethyl acetate to prepare a fiber spinning solution, which is electrospun After silk treatment, vacuum-dry at 45°C for 8 hours to obtain traditional Chinese medicine antibacterial polylactic ...

Embodiment 2

[0028] A preparation method of polylactic acid / hydroxyapatite composite material reinforced by polylactic acid fiber, is characterized in that, comprises the following steps:

[0029] (1) Dried Scutellaria baicalensis and honeysuckle were crushed through a 60-mesh sieve, and the two kinds of traditional Chinese medicine powders were mixed according to the mass ratio of 1:1.2. After microwave treatment for 12 minutes, the traditional Chinese medicine powder was mixed with 45% ethanol-water mixture by 1 : After mixing with a mass volume ratio (g / mL) of 17, reflux extraction at 65°C for 3 hours and then filter, pass the filtrate through an ultrafiltration membrane with a molecular weight cut-off of 8000, spin dry, crush and sieve to obtain a natural antibacterial agent;

[0030] (2) Mix 15 parts of polylactic acid, 0.15 parts of natural antibacterial agent, 0.1 part of gallic acid, 44 parts of N,N-dimethylformamide, and 40.75 parts of ethyl acetate to prepare a fiber spinning solu...

Embodiment 3

[0035] A preparation method of polylactic acid / hydroxyapatite composite material reinforced by polylactic acid fiber, is characterized in that, comprises the following steps:

[0036] (1) Dried Scutellaria baicalensis and honeysuckle were crushed through a 60-mesh sieve, and the two kinds of traditional Chinese medicine powders were mixed according to the mass ratio of 1:0.8. After microwave treatment for 12 minutes, the traditional Chinese medicine powder was mixed with 55% ethanol-water mixture by 1 : After mixing with a mass volume ratio (g / mL) of 17, reflux extraction at 65°C for 3 hours and then filter, pass the filtrate through an ultrafiltration membrane with a molecular weight cut-off of 8000, spin dry, crush and sieve to obtain a natural antibacterial agent;

[0037] (2) Mix 15 parts of polylactic acid, 0.15 parts of natural antibacterial agent, 0.1 part of gallic acid, 35 parts of N,N-dimethylformamide, and 49.75 parts of ethyl acetate to prepare a fiber spinning solu...

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Abstract

The invention belongs to a preparation and application technology of novel-function polymer materials of polymer materials in novel materials, and relates to the technical field of modified plastic, in particular to a preparation method of a polylactic acid fiber reinforced polylactic acid / hydroxyapatite composite material. The preparation method comprises the steps that firstly, active ingredients are extracted from radix scutellariae and honeysuckle flowers to be used as natural antibacterial agents; then electrostatic spinning treatment is carried out on polylactic acid, the natural antibacterial agents and gallic acid to obtain traditional Chinese medicine antibacterial polylactic acid fibers; hydroxyapatite-chitosan-SiO2 hybrid sol is prepared from chitosan, Ca(NO3)2, H3PO4 and silicon dioxide sol, which are taken as raw materials, and freezing, drying and smashing are conducted to obtain a hydroxyapatite-chitosan-SiO2 hybrid; and finally, after the antibacterial polylactic acid fibers and the hydroxyapatite-chitosan-SiO2 hybrid are evenly mixed, master batch is prepared after extrusion and pelleting, and then the surface of the master batch is modified with polylactic acid toobtain the polylactic acid fiber reinforced polylactic acid / hydroxyapatite composite material.

Description

technical field [0001] The invention belongs to the preparation and application technology of novel functional polymer materials of polymer materials in new materials, and relates to the technical field of modified plastics, specifically a polylactic acid / hydroxyapatite composite material reinforced with polylactic acid fibers and its preparation method. Background technique [0002] Polylactic acid (PLA), also known as polylactide, has been widely used in the biomedical industry due to its excellent degradability and biocompatibility as well as its non-toxic and non-irritating properties. However, polylactic acid also has insufficient mechanical strength, and the degradation products are acidic, which can cause inflammatory reactions in the body. Hydroxyapatite (HA) is the main inorganic component of human bone tissue, can induce bone growth, and is a good filling material for bone defect repair. However, due to its poor mechanical strength and fatigue strength, high brit...

Claims

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Application Information

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IPC IPC(8): C08L67/04C08K9/04C08K9/02C08K3/32C08J3/22D01F6/92D01F1/10
CPCC08J3/226C08J2367/04C08J2467/04C08K9/02C08K9/08C08K2003/325D01F1/103D01F6/92
Inventor 林毅平
Owner 林毅平