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A method for separating and recovering mixed heavy metals using calcium alginate membrane

A technology of calcium alginate and heavy metals, applied in the field of resources and environment, and functional materials, can solve the problems of serious heavy metal pollution, heavy metal pollution, and difficulty in separation and recovery of heavy metals. The method is simple, the removal efficiency and recovery efficiency are high, and the application prospect is good. Effect

Inactive Publication Date: 2020-04-24
TIANJIN POLYTECHNIC UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0006] In view of the deficiencies in the prior art, the technical problems to be solved by the present invention are serious heavy metal pollution, low efficiency of alginate adsorption of heavy metal ions, difficulty in separation and recovery of heavy metals after adsorption, etc.
[0007] The technical scheme of the present invention to solve the problems of serious heavy metal pollution, low efficiency of alginate adsorption of heavy metal ions, and difficulty in separation and recovery of heavy metals after adsorption is to provide a method for separating and recovering mixed heavy metals using calcium alginate membranes

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0018] a) Weigh 0.5g of sodium alginate, weigh 1% urea by mass of sodium alginate, dissolve it in 50mL of deionized water under stirring to obtain an aqueous solution of sodium alginate, and obtain a casting solution after defoaming;

[0019] b) preparing a 0.5% calcium chloride aqueous solution as an ion cross-linking agent in a mass percentage of 0.5%;

[0020] c) Take 1 g of the casting solution obtained in step a) and pour it on a clean and flat glass plate, scrape it into a liquid film with a uniform thickness with a scraper rod with a thickness of 100 μm, and immediately soak the liquid film and the glass plate into step b) In the obtained ionic cross-linking agent, soak for 0.5 hour to obtain a calcium alginate film, and soak in an aqueous calcium chloride solution for use;

[0021] d) prepare an aqueous solution of lead ions and iron ions, the mass percentage of each heavy metal ion is 0.01%, and the pH value of the solution is adjusted to 3.0 with dilute nitric acid; ...

Embodiment 2

[0024] a) Weigh 2 g of sodium alginate, weigh polyethylene glycol with a mass percentage of sodium alginate of 150%, and dissolve it in 100 mL of deionized water under stirring to obtain an aqueous solution of sodium alginate, and obtain a casting solution after defoaming;

[0025] b) preparing an aqueous calcium nitrate solution with a mass percentage of 50% as an ion cross-linking agent;

[0026] c) Take 5 g of the casting solution obtained in step a) and pour it on a clean and flat glass plate, scrape it into a liquid film with a uniform thickness with a scraper rod with a thickness of 1000 μm, and immediately soak the liquid film and the glass plate into step b) In the obtained ionic cross-linking agent, soak for 24 hours to obtain a calcium alginate film, and soak in an aqueous calcium chloride solution for use;

[0027] d) prepare an aqueous solution of copper ions and cadmium ions, the mass percentage of each heavy metal ion is 10%, and the pH value of the solution is a...

Embodiment 3

[0030]a) Weigh 1 g of sodium alginate, weigh polyvinylpyrrolidone with a mass percentage of sodium alginate of 50%, and dissolve it in 80 mL of deionized water under stirring to obtain an aqueous solution of sodium alginate, and obtain a casting solution after defoaming;

[0031] b) preparing a 5% calcium dihydrogen phosphate aqueous solution as an ion cross-linking agent;

[0032] c) Take 2g of the casting solution obtained in step a) and pour it on a clean and flat glass plate, scrape it into a liquid film with a uniform thickness with a scraper rod with a thickness of 500 μm, and immediately soak the liquid film and the glass plate into step b) In the obtained ionic cross-linking agent, soak for 8 hours to obtain a calcium alginate film, and soak in an aqueous calcium chloride solution for use;

[0033] d) preparing an aqueous solution of lead ions, copper ions and cadmium ions, the mass percentage of each heavy metal ion is 1%, and the pH value of the solution is adjusted ...

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PUM

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Abstract

The invention provides a method for separating and recovering mixed heavy metals by using a calcium alginate film. The method comprises the following steps: dissolving sodium alginate in water to obtain a film casting solution, and then controlling the thickness of a film scraping rod and performing calcium ion cross-linking so as to obtain calcium alginate hydrogel films with different thicknesses; preparing mixed aqueous heavy metal ion solutions with different concentrations, and then performing filtering with the mixed aqueous heavy metal ion solutions as feed liquids and the calcium alginate hydrogel films as filtering films so as to separate different heavy metal ions in virtue of difference between exchange capacities of calcium alginate and different heavy metal ions; and subjecting the heavy metal ions retained on the calcium alginate hydrogel films to alkali-liquor hydrothermal treatment, filtering and firing so as to obtain recovered heavy metal oxides. The method of the invention is simple in process, free of usage of any organic solvent, friendly to environment and high in heavy metal removal efficiency and recovery efficiency, and has good application prospects.

Description

technical field [0001] The invention relates to a method for separating and recovering mixed heavy metals by using a calcium alginate membrane, and belongs to the fields of functional materials, resources and environment. Background technique [0002] Water sources and soils polluted by heavy metals have been considered to be serious and persistent environmental problems. Heavy metals are not biodegradable and accumulate in ecosystems as well as in humans. Lead, copper and cadmium are three common types of heavy metals in industrial wastewater. Lead is toxic to the human body, and it can interact with the sulfhydryl group of the protein, thereby causing the destruction of the metabolic activity and biological activity of the protein. Copper can cause various types of acute and chronic conditions in humans, such as hemochromatosis and gastrointestinal mucositis. Cadmium accumulation in humans can cause unexpected diseases and renal abnormalities, including prourokinase and...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B01D71/08B01D67/00C02F1/44C02F1/42C22B7/00C08J3/24C02F101/20C08L5/04
CPCB01D67/0006B01D71/08B01D2323/30C02F1/42C02F1/44C02F2001/425C02F2101/20C02F2301/08C08J3/24C08J2305/04C22B7/006Y02P10/20
Inventor 赵孔银刘亮许国庆苏虹娴赵磊张璐张可叶昀
Owner TIANJIN POLYTECHNIC UNIV