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Method for recovering valuable metal from battery electrode material leaching liquid

A technology of valuable metals and battery electrodes, which is applied in the field of recycling valuable metals, can solve problems such as safety pollution and impact on the sustainable development of new energy vehicles, and achieve the effects of saving costs, avoiding cost consumption, and reducing production costs

Inactive Publication Date: 2019-05-28
GUANGDONG INST OF RARE METALS
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

In short, the recycling of power batteries is related to safety, pollution, and resource issues, and also affects the sustainable development of new energy vehicles.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0016] A leach solution of a waste lithium-ion battery electrode material, which contains nickel 5g / L, cobalt 20g / L, aluminum 1.9g / L, manganese 0.10g / L, lithium 10g / L, copper 2g / L, iron 0.1g / L and phosphorus 0.2g / L. Use sodium hydroxide to adjust the pH value of the leaching solution to 0.2, and extract copper with Lix984 extractant at a volume ratio of 1:1 to obtain a raffinate containing iron, aluminum, manganese, nickel, cobalt and lithium, and recover copper from the organic phase containing copper ; Press the molar ratio 1:0.7 of phosphate root and iron and aluminum ion, add the sodium phosphate solution of concentration 0.01mol / L in the raffinate to precipitate iron and aluminum, stir for 3 hours, filter, obtain precipitate and precipitation mother liquor; The volume ratio is 1:1, and the precipitated mother liquor is extracted and separated with P204 extractant to obtain lithium-containing raffinate and manganese-nickel-cobalt organic phase; adding a sulfuric acid solut...

Embodiment 2

[0018] A leach solution of a waste lithium-ion battery electrode material, which contains nickel 5g / L, cobalt 20g / L, aluminum 1.9g / L, manganese 0.10g / L, lithium 10g / L, copper 2g / L, iron 0.1g / L and phosphorus 0.2g / L; use sodium hydroxide to adjust the pH value of the leach solution to 0.9, and extract copper with M5640 extractant at a volume ratio of 5:1 to obtain a raffinate containing iron, aluminum, manganese, nickel, cobalt and lithium, containing copper The organic phase reclaims copper; According to the molar ratio of phosphate root and iron and aluminum ion 1:1, the sodium phosphate solution of concentration 1mol / L is added in the raffinate and precipitates iron and aluminum, stirs 0.5 hour, filters, and obtains precipitate and Precipitation mother liquor; according to the volume ratio of 5:1, extract and separate the precipitation mother liquor with Cyanex272 extractant to obtain lithium-containing raffinate and manganese-nickel-cobalt organic phase; add a concentration ...

Embodiment 3

[0020] A leach solution of a waste lithium-ion battery electrode material contains nickel 38g / L, cobalt 8g / L, aluminum 0.9g / L, manganese 17.0g / L, lithium 3g / L, copper 0.2g / L, iron 2.7g / L and Phosphorus 2.8g / L; Regulate pH value of leaching solution with sodium carbonate to be 2.2, filter to get sediment and filtrate; Regulate pH value of leaching solution with sodium hydroxide to be 0.5, by volume ratio 3:1, extract copper with Lix973 extraction agent, obtain The raffinate containing iron, aluminum, manganese, nickel, cobalt and lithium, and the organic phase containing copper recover copper; according to the molar ratio of phosphate to iron and aluminum ions 1:0.8, the sodium phosphate solution with a concentration of 0.09mol / L Add the raffinate to precipitate iron and aluminum, stir for 2.5 hours, and filter to obtain the precipitate and the precipitated mother liquor; the precipitated mother liquor is extracted and separated with a mixed extractant of P204 and P507 at a volu...

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PUM

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Abstract

The invention discloses a method for recovering valuable metal from battery electrode material leaching liquid. The method comprises the following steps: the pH value of leaching liquid is adjusted; copper is extracted by using an extracting liquid; raffinate containing iron, aluminum, manganese, nickel, cobalt and lithium and an organic phase containing copper are obtained; sodium phosphate solution is fed in the raffinate to precipitate iron and aluminum, is stirred by 0.5-3 hours, and is filtered to obtain precipitates and precipitation mother liquor; the precipitation mother liquor is extracted and separated by acid phosphorus-contained extracting agent to obtain raffinate containing lithium and an organic phase containing manganese, nickel and cobalt; sulfuric acid solution with a concentration of 0.2-3 mol / L is fed in the organic phase containing manganese, nickel and cobalt for reverse extraction to obtain solution containing manganese, nickel and cobalt; the sodium phosphate solution is fed in the raffinate, is stirred by 0.5-3 hours, and is filtered to obtain lithium phosphate and precipitation mother liquor; and precipitates of iron and aluminum are returned from part ofthe precipitation mother liquor. The method recovers manganese, nickel and cobalt from the battery electrode material leaching liquid, reduces the recovery cost, and improves the lithium battery recovery economical benefit.

Description

technical field [0001] The invention belongs to a method for recovering valuable metals from the leaching solution of waste lithium ion battery electrode materials. Background technique [0002] With the rapid development of lithium-ion batteries, lithium-ion batteries have occupied the portable consumer electronics market, and continue to expand to new energy electric vehicles and other fields. my country has become the world's largest producer, consumer and exporter of lithium batteries. It is estimated that by 2020, the demand for power lithium-ion batteries will reach 125Gwh, and the amount of scrap will reach 2.2Gwh, about 500,000 tons. By 2023, the amount of scrap will reach 101Gwh, about 1.16 million tons. In short, power battery recycling is related to safety, pollution, and resource issues, and also affects the sustainable development of new energy vehicles. The development of waste lithium-ion battery recycling technology is not only beneficial to environmental p...

Claims

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Application Information

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IPC IPC(8): C22B7/00C22B15/00C22B21/00C22B26/12H01M10/54C22B23/00C22B3/38C22B47/00
CPCY02P10/20Y02W30/84
Inventor 刘志强王东兴张魁芳饶帅李伟曹洪杨
Owner GUANGDONG INST OF RARE METALS