GSTs quantitative detection device and detection method and application thereof
A quantitative detection method and quantitative detection technology, applied in the biological field, can solve the problems of inability to represent and provide, achieve accurate and stable global detection, and realize the effect of global detection
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Embodiment 1
[0058] Embodiment 1: Preparation of 47 isotope-labeled GSTs family protein peptides
[0059] Forty-seven stable isotope-labeled GSTs family protein peptides with known quantitative information were synthesized.
[0060] Table 1
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[0062]
[0063]
[0064] Note: [+1] indicates that the detected peptide has natural deamination at this amino acid, so the molecular weight increases by 1;
[0065] Table 2
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[0067]
Embodiment 2
[0068] Example 2: Sample preparation of low-abundance GSTs in plasma
[0069] The low-abundance GSTs sample preparation method in the plasma comprises the following steps:
[0070] 1) Preparation of plasma samples
[0071] (1) Collect whole blood samples into 5mL vacuum EDTA-K2 blood collection tubes, slowly invert and mix well and let stand;
[0072] (2) Place the blood collection tube in a pre-cooled centrifuge, centrifuge at 2000g for 30min at 4°C, and separate the plasma;
[0073] (3) Carefully take out the blood collection tube and place it on ice to keep the temperature low, and observe whether the centrifuged sample has hemolysis. If the sample has hemolysis, the sample cannot be used for subsequent experiments;
[0074] (4) Carefully draw the upper layer of plasma and transfer it to a clean 1.5mL EP tube, and fill each tube with 600μL of plasma;
[0075] (5) The aliquoted plasma samples were frozen and stored at -80°C for later use.
[0076] 2) Affinity enrichment ...
Embodiment 3
[0104] Embodiment 3: the preparation of standard curve
[0105] Add 47 stable isotope-labeled GSTs family protein peptides with known quantitative information according to the concentration of Example 1 (wherein the concentration is the average concentration of the target peptide in the sample mixed with all samples when the standard curve is prepared) In the prepared mixed sample of plasma GSTs enzymatic hydrolysis, the obtained mixed sample was quantitatively detected by using the PRM mode to detect 47 stable isotope-labeled peptides and endogenous peptides in the sample. The specific detection conditions are as follows: after injection, the sample Under the condition of mobile phase A of 5 μL / min, the trap column was first enriched for 5 minutes, and then the peptides were eluted and separated according to the procedures in Table 3. The ions entering the mass spectrometer were detected in PRM mode. For basic PRM parameter settings, see Table 4 shows.
[0106] table 3
[0...
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