Unlock instant, AI-driven research and patent intelligence for your innovation.

A method for improving the rheological properties of coal tar pitch

A technology of rheological properties and coal tar pitch, applied in the processing of tar pitch/petroleum pitch/natural pitch, processing tar pitch/petroleum pitch/natural pitch by distillation, processing tar pitch/petroleum pitch/natural pitch by chemical methods, etc. , can solve the problems of not mentioning the recycling of hydrogenation reagents, the large amount of hydrogenation reagents used, and the high cost, and achieve the effects of increasing application value, reducing production costs, and reducing softening point

Active Publication Date: 2022-07-08
WUHAN UNIV OF SCI & TECH
View PDF11 Cites 0 Cited by
  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Chinese patent CN106947525A mentions a method for adsorption and removal of heteroatoms, but only nitrogen heteroatoms and sulfur heteroatoms are removed
[0006] In the existing methods disclosed above, the use of hydrogenation reagents is large and the recycling of hydrogenation reagents is not mentioned, resulting in high cost of coal tar pitch hydrogenation process

Method used

the structure of the environmentally friendly knitted fabric provided by the present invention; figure 2 Flow chart of the yarn wrapping machine for environmentally friendly knitted fabrics and storage devices; image 3 Is the parameter map of the yarn covering machine
View more

Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0027] A method for improving the rheological properties of coal tar pitch, comprising the following steps in turn:

[0028] (1) Add the hydrogen donor and coal tar pitch into the autoclave together according to the mass ratio of 1:19, close the autoclave and keep the reactor sealed; wherein, the softening point of coal tar pitch is 92°C, and the mass content of nitrogen element is 1.3% , the mass content of sulfur element is 0.6%, the mass content of oxygen element is 2.3%; the hydrogen donor is tetralin;

[0029] (2) Adjust the heating procedure of the autoclave, so that the materials in the autoclave are heated to 420°C at room temperature for 3 hours, and the hydrogenation reaction is carried out at a constant temperature of 420°C for 8 hours. After the temperature of the material in the kettle dropped to 280°C, and kept at a constant temperature for 10 hours, the residual hydrogen-donating agent was recovered by vacuum distillation. During the vacuum distillation process,...

Embodiment 2

[0033] A method for improving the rheological properties of coal tar pitch, comprising the following steps in turn:

[0034] (1) Add the hydrogen donor and coal tar pitch into the autoclave together according to the mass ratio of 6:5, close the autoclave and keep the reactor sealed; wherein, the softening point of coal tar pitch is 92°C, and the mass content of nitrogen element is 1.3% , the mass content of sulfur element is 0.6%, the mass content of oxygen element is 2.3%; the hydrogen donor is decalin;

[0035](2) Adjust the heating procedure of the autoclave so that the materials in the autoclave are heated to 440°C at room temperature for 3 hours, and the hydrogenation reaction is carried out at a constant temperature of 440°C for 8 hours. When the temperature of the material in the kettle is 300°C, the residual hydrogen-donating agent is recovered by vacuum distillation. During the vacuum distillation process, the pressure in the kettle is 0 MPa, and the constant temperat...

Embodiment 3

[0039] A method for improving the rheological properties of coal tar pitch, comprising the following steps in turn:

[0040] (1) Add the hydrogen donor and coal tar pitch into the autoclave together according to the mass ratio of 6:5, close the autoclave and keep the reactor sealed; wherein, the softening point of coal tar pitch is 92°C, and the mass content of nitrogen element is 1.3% , the mass content of sulfur element is 0.6%, the mass content of oxygen element is 2.3%; the hydrogen donor is tetrahydroquinoline;

[0041] (2) Adjust the heating procedure of the autoclave, so that the materials in the autoclave are heated at room temperature for 3 hours to reach 450 °C, and the hydrogenation reaction is carried out at a constant temperature of 450 °C for 12 hours. ; When the temperature of the material in the kettle drops to 150 °C, the residual hydrogen-donating agent is recovered by vacuum distillation. During the vacuum distillation process, the pressure in the kettle is ...

the structure of the environmentally friendly knitted fabric provided by the present invention; figure 2 Flow chart of the yarn wrapping machine for environmentally friendly knitted fabrics and storage devices; image 3 Is the parameter map of the yarn covering machine
Login to View More

PUM

PropertyMeasurementUnit
softening pointaaaaaaaaaa
softening pointaaaaaaaaaa
softening pointaaaaaaaaaa
Login to View More

Abstract

The invention relates to a method for improving the rheological properties of coal tar pitch. It sequentially includes the following steps: (1) adding the hydrogen-donating agent and coal pitch into the autoclave in a certain mass ratio, fully mixing, and sealing the reaction kettle; (2) heating the material in the kettle to 350-450°C, keeping the The hydrogenation reaction is carried out at a constant temperature; after that, the temperature of the material in the kettle drops to 200-320 °C, and the pressure is released; the residual hydrogen donor is recovered by vacuum distillation, and then cooled to room temperature; during the hydrogenation reaction and the vacuum distillation process, the reaction kettle Keep stirring; (3) reheat the coal tar pitch obtained by the treatment to 420° C. and keep the constant temperature for 2-10 hours. The method can control the content of heteroatoms in coal tar pitch and improve its rheological properties at the same time.

Description

technical field [0001] The invention relates to the modification treatment and application of coal tar pitch, in particular to a method for improving the rheological properties of coal tar pitch. Background technique [0002] Coal tar is one of the main by-products in the coal coking process. Coal tar, as the bottom product of coal tar distillation, accounts for about 55% to 65% of coal tar or even more. my country is rich in coal resources. In 2018, the national coal tar output was 18.06 million tons, the operating rate of the coal tar deep processing industry was about 50%, and the coal tar pitch was about 6.818 million tons. Nearly half of the production capacity was idle. In the past, coal tar pitch was mainly used in low-value-added fields such as coatings, paving asphalt, and binders. In recent years, with the improvement of the country's environmental protection requirements, coupled with the continuous development of high-value-added applications for by-products such...

Claims

the structure of the environmentally friendly knitted fabric provided by the present invention; figure 2 Flow chart of the yarn wrapping machine for environmentally friendly knitted fabrics and storage devices; image 3 Is the parameter map of the yarn covering machine
Login to View More

Application Information

Patent Timeline
no application Login to View More
Patent Type & Authority Patents(China)
IPC IPC(8): C10C3/02C10C3/06
CPCC10C3/023C10C3/06
Inventor 李轩科李重郭建光
Owner WUHAN UNIV OF SCI & TECH