Titanium dioxide paste, porous semiconductor electrode substrate, photoelectrode, and dye-sensitized photovoltaic cell
A titanium dioxide, semiconductor technology, applied in the direction of titanium dioxide, titanium oxide/hydroxide, photosensitive equipment, etc.
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Embodiment 1
[0167]
[0168] Titanium dioxide nanoparticles A (average particle diameter: 30nm) are added to an aqueous sol (solid content concentration: 18% to 20% by mass, pH 2.6) obtained by dispersing titanium dioxide nanoparticles D (average particle diameter: 12nm) in water and the powder of titanium dioxide nanoparticles B (average particle diameter: 40 nm) were mixed so that the mass ratio in terms of solid content was A:B:D=47:30:23. In addition, the average particle diameter of titanium dioxide nanoparticle A and B is the value calculated by the particle diameter distribution measurement obtained by the scanning electron microscope observation method. Further, ethylene glycol mono-tert-butyl ether (EGTBE) and diacetone alcohol (DAA) were added so that the concentrations in the titanium dioxide paste became EGTBE: 4.8% by mass and DAA: 1.9% by mass, respectively, to obtain a mixture. The mixture was dispersed by passing through a table-top three-roll mill 10 times to prepare a t...
Embodiment 2
[0182] In the preparation of the titanium dioxide paste of Example 1, by changing the pH of the aqueous sol containing titanium dioxide nanoparticles D from 2.6 to 2.9, the pH of the obtained titanium dioxide paste was changed from 2.9 to 3.1, in addition, the same as in Example 1 In the same manner, a titanium dioxide paste, a porous semiconductor electrode substrate, and a dye-sensitized solar cell were prepared or produced, and various measurements and evaluations were performed. The results are shown in Table 1.
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