High-quality silicon carbide seed crystal, silicon carbide crystal, silicon carbide substrate and preparation method thereof
A technology of high-quality silicon carbide seeds and silicon carbide seeds, applied in chemical instruments and methods, crystal growth, single crystal growth, etc., can solve problems such as poor quality of silicon carbide substrates and affecting applications
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[0113] About the preparation method of silicon carbide seed crystal :
[0114] The present invention provides a method for preparing a high-quality silicon carbide seed crystal described in the above technical solution, comprising the following steps:
[0115] a) performing the first diameter expansion growth on the primary seed crystal to obtain the primary growth crystal;
[0116] b) processing the primary growth crystal to obtain an intermediate seed crystal containing only diameter-expanding regions;
[0117] c) Performing a second diameter-expanding growth on the intermediate seed crystal to obtain a high-grade seed crystal.
[0118] With regard to step a): the primary seed crystal is first expanded in diameter to obtain a primary growth crystal.
[0119] In the present invention, the type and source of the primary seed crystal are not particularly limited, and it can be a general commercially available SiC seed crystal; the commercially available seed crystal usually...
Embodiment 1
[0243] Example 1: Preparation of SiC seed crystal
[0244] S1. Provide primary seeds: micropipe density 2 / cm 2 , screw dislocation density 1000 / cm 2 , compound dislocation density 50 / cm 2 .
[0245] S2. Carry out the first diameter expansion growth: select the diameter expansion angle as 45°; control the axial temperature gradient in the growth chamber: along the crystal growth direction, the temperature gradually increases from the surface of the seed crystal to the surface of the silicon carbide raw material, and the temperature gradient is 2 °C / cm; the lateral temperature gradient is: the temperature gradually increases from the center of the seed crystal along the radial direction to the edge of the seed crystal, and the temperature gradient is 2°C / cm.
[0246] S3. Cutting the crystal grown in step S2 to obtain an intermediate seed crystal containing an equal diameter region and an enlarged diameter region. It is then processed to obtain a high-quality intermediate see...
Embodiment 2
[0251] Embodiment 2: Preparation of silicon carbide powder
[0252] S1. Graphite powder pretreatment: Put high-purity graphite powder (total impurity content < 10ppm) into a high-temperature furnace, evacuate the furnace and keep the vacuum pump unit working all the time, then raise the temperature in the furnace to 2250°C and keep it for 10 hours; During the above heat preservation process, first turn off the vacuum pump unit, fill it with argon to 50000Pa and keep it for 10 minutes, then turn on the vacuum pump to evacuate the furnace again and keep the vacuum pump unit working all the time. Obtain pretreated graphite powder.
[0253] The boron impurity content of gained pretreatment graphite powder is 5.5 * 10 15 / cm 3 , the aluminum impurity content is 4×10 14 / cm 3 .
[0254] S2. Mix silicon powder and pretreated graphite powder at a mass ratio of 1.00:1, put them into a graphite crucible in a high-temperature furnace, then evacuate the furnace, and then fill the fur...
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