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Preparation method of high-quality spinning pitch, product and application of high-quality spinning pitch

A high-quality, spinning technology, used in textiles and papermaking, fiber chemical characteristics, etc., can solve the problems of severe reaction conditions, low yield, low product purity, etc., and achieve mild reaction conditions, high safety factor, and high reactivity. Effect

Pending Publication Date: 2021-11-09
WUHAN UNIV OF SCI & TECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0009] From the above analysis, it can be seen that there are problems such as high raw material cost, severe reaction conditions, low yield and low product purity in the existing method for preparing mesophase pitch, which makes the spinning performance of the prepared pitch poor and cannot be achieved in specific applications. very good result

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0044] Add 300mL of toluene, 14.38g of liquid bromine, and 21.33g of 1-methylnaphthalene (the molar ratio of 1-methylnaphthalene to the brominating agent is 1.7:1) in a 500mL three-necked flask in sequence. Nitrogen was used as a protective atmosphere, and the nitrogen flow rate was 50 mL / min. The reactants were placed in a constant temperature water bath at 50° C. to preheat them, and magnetic stirring was used to ensure that the reactants were evenly mixed. When the temperature of the reaction material rises to 50° C., continue to maintain the magnetic stirring state, and turn on the xenon lamp (300w) to carry out the photocatalytic reaction for 6 hours. After the reaction is completed, the product is suction filtered, washed with water, distilled under reduced pressure, and dried to obtain 1-bromomethylnaphthalene. The yield and selectivity of 1-bromomethylnaphthalene were measured by GC-MS, and the results showed that the yield of 1-bromomethylnaphthalene could reach 94%, ...

Embodiment 2

[0047] Add 300mL of benzene, 14.38g of liquid bromine, and 21.33g of 1-methylnaphthalene (the molar ratio of 1-methylnaphthalene to the brominating agent is 1.7:1) into a 500mL three-necked flask in sequence. Nitrogen was used as a protective atmosphere, and the nitrogen flow rate was 50 mL / min. The reactants were placed in a constant temperature water bath at 50° C. to preheat them, and magnetic stirring was used to ensure that the reactants were evenly mixed. When the temperature of the reaction material rises to 50° C., continue to maintain the magnetic stirring state, and turn on the xenon lamp (300w) to carry out the photocatalytic reaction for 5 hours. After the reaction is completed, the product is suction filtered, washed with water, distilled under reduced pressure, and dried to obtain 1-bromomethylnaphthalene. The yield and selectivity of 1-bromomethylnaphthalene were measured by GC-MS, and the results showed that the yield of 1-bromomethylnaphthalene could reach 96%...

Embodiment 3

[0050] Add 300mL of carbon tetrachloride, 12.53g of boron tribromide, and 21.33g of 2-methylnaphthalene (the molar ratio of 2-methylnaphthalene to brominating agent is 3:1) in sequence in a 500mL three-necked flask. Nitrogen gas was introduced into the reaction system as a protective atmosphere, and the flow rate of nitrogen gas was 75mL / min. The reactant was placed in a constant temperature water bath at 60°C to preheat it, and magnetic stirring was used to ensure that the reaction material was evenly mixed. When the temperature of the reaction material rises to 60° C., continue to maintain the state of magnetic stirring, and turn on the xenon lamp (300w) to carry out the photocatalytic reaction for 4 hours. After the reaction is completed, the product is suction filtered, washed with water, distilled under reduced pressure, and dried to obtain 2-bromomethylnaphthalene. The yield and selectivity of 2-bromomethylnaphthalene were determined by GC-MS, and the results showed that...

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Abstract

The invention discloses a preparation method of high-quality spinning asphalt, and a product and application of the high-quality spinning asphalt, and belongs to the field of high-quality synthetic asphalt. The method comprises the following steps: sequentially adding a brominating agent, methylnaphthalene and a solvent under the protection of a nitrogen atmosphere, mixing, carrying out photocatalytic reaction at a temperature of 40-70 DEG C, and carrying out suction filtration, washing, reduced pressure distillation and drying to obtain brominated methylnaphthalene; and under the protection of a nitrogen atmosphere, carrying out heat treatment on the obtained brominated methylnaphthalene at 200-350 DEG C for 6-12 hours, compensating the brominated methylnaphthalene, carrying out heat treatment under the same condition for 3-6 hours, and extracting to obtain the high-quality spinning pitch. Compared with the prior art, the method of the invention has the following characteristics that the raw materials for preparing the precursor of the asphalt are cheap and easy to obtain, the condition is mild, the product is single, the asphalt prepared from the precursor has the advantages of excellent spinnability, narrow molecular weight distribution, good melt fluidity and the like, and the preparation of high-performance asphalt-based carbon fibers is facilitated.

Description

technical field [0001] The invention relates to the technical field of high-quality synthetic asphalt, in particular to a preparation method of high-quality spinning asphalt and its product and application. Background technique [0002] In recent years, the continuous increase of automobile production and ownership has exacerbated problems in energy, environment, safety and other aspects. Energy conservation and environmental protection have become the primary issues facing the global auto industry. Under the current situation, to realize the sustainable development of the automobile industry, it is necessary to develop new technologies for energy saving and emission reduction to reduce the energy consumption of automobiles and the environmental pollution produced. Studies have shown that vehicle lightweight is one of the most effective measures to reduce energy consumption and emissions. Automobile lightweight can be achieved through lightweight materials, lightweight str...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): C08G61/02D01F9/145
CPCC08G61/02D01F9/145C08G2261/11C08G2261/1412C08G2261/314C08G2261/3326C08G2261/93
Inventor 董志军刘金港李轩科田永胜袁观明李保六郭建光柯昌美
Owner WUHAN UNIV OF SCI & TECH