Pellicle membrane
a technology of pellicle membrane and pellicle, which is applied in the field of pellicle membrane, can solve the problems of cumbersome and complicated manufacturing process of pellicle membrane, and achieve the effect of simple manufacturing and long-term maintenance of patterning precision
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[0067]The present invention will now be described in more detail with reference to Examples, which however shall not be construed as limiting the scope of the present invention.
examples 1to 7
,Comparative Examples 1to 4
[0068]An amorphous fluoropolymer CYTOP (code: CHX809SP2, Asahi Glass, Co., Ltd.) was dissolved into a fluorine-containing solvent perfluorotributylamine (EFL-174S, Tohkem Products, Corporation) to afford a solution containing 6wt % polymer. The solution thus obtained was filtrated through a polytetrafluoroethylene (PTFE) membrane filter (pore size: 500nm) to afford a filtrate deprived of foreign material.
[0069]The filtrate thus obtained was applied onto a surface of a quarts glass substrate (25cm×25cm) by spin coating (spin speed: 700 rpm, spin time: 60seconds) to deposit a coated film.
[0070]The coated film formed on the substrate surface was heated to 165° C. in a clean oven. The heating time was adjusted as shown in Table 1below (in the range of 80to 400seconds) to produce a dried film. After drying, a resin-made peeling ring was attached to the dried film on the substrate surface, and the dried film was peeled off the substrate to provide a pellicle mem...
examples 8to 11
, Comparative Example 7
[0091]Pellicle membranes were prepared in the same manner as in Example 1except that the spin coating condition was changed and that the drying temperatures and drying times given in Table 2were used. The pellicle membranes obtained had a thickness of 281nm. In the same manner as in Example 1, the fluorine-containing solvent contained in the pellicle membrane was gasified, and the amount of the gasified fluorine-containing solvent was measured. The fluorine-containing solvent contents are given in Table 2.
[0092]
TABLE 2Drying temp.Drying timeFluorine-based solvent content(° C.)(sec)(ppm by weight)Comp. Ex. 7165380 3Ex. 8165350 7Ex. 916532013Ex. 1016529016Ex. 1116526027
[0093]Each of the pellicle membranes prepared in Example 11and Comparative Example 7was irradiated with ArF excimer laser in the same manner as in Example 1. The irradiation density was set to 1 mJ / cm2 / pulse, and laser oscillation frequency to 500Hz.
[0094]The graph shown in FIG. 4 is a graph of re...
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