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Method for increasing yield of propylene

A technology of propylene and ethylene, which is applied in the field of olefin catalytic cracking technology to improve the yield of propylene, and can solve the problems of low selectivity and low yield of propylene

Active Publication Date: 2008-04-23
CHINA PETROLEUM & CHEM CORP +1
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0008] The technical problem to be solved by the present invention is that there are low yield and low selectivity of the target product propylene in the prior literature and technology, and a new method for improving the propylene yield is provided

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0015] Using methanol as raw material, the first reactor adopts a fluidized bed reactor with SAPO-34 molecular sieve as a catalyst, the second reactor adopts a fixed bed reactor with tungsten oxide as a catalyst, and the third reactor adopts a fixed bed reactor. Using ZSM-5 molecular sieve as the catalyst, the reaction temperature of the first reactor is 450°C, and the reaction space velocity is 6 hours -1 , the reaction pressure is 0.1MPa; the reaction temperature of the second reactor is 300°C, and the reaction space velocity is 1 hour -1 , the mass ratio of ethylene to butene is 1:1, and the reaction pressure is 3MPa. The reaction temperature of the third reactor is 480°C, and the reaction space velocity is 8 hours -1 , the pressure is 0.1MPa. In the experiment, after the reaction products in the first reactor were separated, all butene-1 and butene-2 ​​entered the second reactor for reaction, and the remaining carbon four and above hydrocarbons entered the third reactor ...

Embodiment 2

[0017] Using dimethyl ether as raw material, the first reactor adopts a fluidized bed reactor with SAPO-34 molecular sieve as a catalyst, the second reactor adopts a fixed bed reactor with tungsten oxide as a catalyst, and the third reactor adopts a fixed bed reaction device, with ZSM-5 molecular sieve as the catalyst, the reaction temperature of the first reactor is 550°C, and the reaction space velocity is 40 hours -1 , the reaction pressure is 0.5MPa; the reaction temperature of the second reactor is 530°C, and the reaction space velocity is 10 hours -1 , the mass ratio of ethylene to butene is 1:1, and the reaction pressure is 0.01MPa. The reaction temperature of the third reactor is 570°C, and the reaction space velocity is 20 hours -1 , the reaction pressure is 0.01MPa. In the experiment, after the reaction products of the first reactor were separated, butene-1 and butene-2 ​​all entered the second reactor for reaction, and the remaining carbon four and above hydrocarb...

Embodiment 3

[0019] Dimethyl ether is used as raw material, water is used as diluent, the mass ratio of dimethyl ether to water is 1:2, the first reactor adopts fluidized bed reactor, SAPO-34 molecular sieve is used as catalyst, and the second reactor adopts fixed The bed reactor uses tungsten oxide as the catalyst, the third reactor uses a fixed bed reactor, uses ZSM-5 molecular sieve as the catalyst, the reaction temperature of the first reactor is 630°C, and the space velocity is 25 hours -1 , the reaction pressure is 1.2MPa; the reaction temperature of the second reactor is 450°C, and the reaction space velocity is 5 hours -1 , the mass ratio of ethylene to butene is 1:1, and the reaction pressure is 0.2MPa. The reaction temperature of the third reactor is 600°C, and the reaction space velocity is 40 hours -1 , the reaction pressure is 1.5MPa. In the experiment, after the reaction products of the first reactor were separated, butene-1 and butene-2 ​​all entered the second reactor for...

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PUM

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Abstract

The present invention relates to one kind of propylene producing process with high selectivity and high yield. The production process includes the following steps: 1. reaction of oxygen compound material in the first reaction region through contacting with catalyst I to produce effluent I containing ethylene, propylene and butylene; and separating the effluent I to obtain ethylene, propylene, butylene-1, butylene-2 and other C4 and C4+ hydrocarbons; 2. reaction of ethylene, butylene-1 and / or butylene-2 in the second reaction region through contacting with catalyst II to produce effluent II containing propylene; and 3. reaction of C4 and C4+ hydrocarbons in the third reaction region through contacting with catalyst III to produce effluent III containing ethylene and propylene. The production process may be applied in industrial production.

Description

technical field [0001] The invention relates to a method for increasing the yield of propylene, in particular to a method for improving the yield of propylene by catalytic reaction of methanol or dimethyl ether, complex butene and ethylene metathesis and olefin catalytic cracking technology. Background technique [0002] Petrochemical industry is an important pillar industry in the national economy. It provides a large amount of chemical raw materials for industry, agriculture, transportation and national defense. It is one of the most relevant and leading industrial sectors in the national economy. Propylene and ethylene are the two most important basic raw materials for modern petrochemical industry. [0003] Propylene is mainly used to produce polypropylene, cumene, carbonyl alcohol, acrylonitrile, propylene oxide, acrylic acid, isopropanol, etc. Among them, polypropylene accounts for more than half of the world's propylene demand. At present, 67% of the world's propylen...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): C07C1/20C07C11/04C07C11/06
CPCY02P20/52Y02P30/20Y02P30/40
Inventor 谢在库刘俊涛杨为民钟思青
Owner CHINA PETROLEUM & CHEM CORP