Aromatic aza allyl organic zinc compound and synthetic method thereof
A technology of heteroallyl and synthesis method, applied in the field of aromatic azaallyl organozinc compounds and synthesis thereof, can solve the problems of harsh synthesis conditions, complex synthesis methods, easy deactivation and the like, and achieves mild and good reaction conditions. Catalytic effect, simple step effect
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[0021] Example 1, the synthesis and characterization of the aromatic azaallyl-containing organozinc compound of the present invention
[0022] (1) Under the protection of nitrogen and ice-water bath, respectively add 0.98g (10mmol) benzyllithium and 1.3ml (10mmol) trimethylchlorosilane to about 30ml n-hexane in turn, stir, naturally warm up to room temperature, keep Stir the reaction for 15 hours, filter the precipitated lithium chloride, and remove the solvent with a vacuum pump to obtain liquid α-(trimethylsilyl)toluene. α-(trimethylsilyl)toluene can be purified by vacuum distillation;
[0023] (2) Under the protection of nitrogen and ice-water bath, 1.71g (10mmol) α-(trimethylsilyl)toluene, 5.6ml1.8M n-butyllithium solution and 1.5ml (10mmol)Me 2 NCH 2 CH 2 NMe 2 (commonly known as tetramethylethylenediamine, lithium salt depolymerization agent) sequentially added to about 30ml of n-hexane, stirred, naturally warmed to room temperature, kept stirring for 15 hours to obt...
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