Freezeproof polypeptide, synthesis, composition containing same and application thereof
A technology of polypeptide composition and antifreeze polypeptide, applied in the biological field, can solve problems such as unfavorable industrialized large-scale production, biological methods are time-consuming and laborious, and cannot repeat experiments, and achieve the effects of excellent antifreeze effect, excellent effect and high yield
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Embodiment 1
[0059] Embodiment 1, the preparation of antifreeze peptide
[0060] 1. Main reagents
[0061] Analytical pure acetylgalactosamine (GalNAc), BF 3 .Et 2 O, SnCl 4 , CH 2 Cl 2 , acetic anhydride and chromatographically pure CH 3 CN was purchased from Sigma; Fmoc-Thr-OH, Fmoc-Ala-OH, and Fmoc-Asn(Trt)-OH monomers were purchased from Advanced ChemTech; RinkAmide resin was purchased from Tianjin Nankai Hecheng Technology Co., Ltd.
[0062] 2. Experimental method
[0063] 2.1 Acetylgalactosamine peracetylation:
[0064]
[0065] a SnCl 4 , Ac 2 O, CH 2 Cl 2 Yield: 52%
[0066] Add 1.5g GalNAc, 15ml CH 2 Cl 2 , 15ml acetic anhydride and 120mg SnCl 4 , after reflux reaction at 50°C for 12 hours, it was separated by a normal phase silica gel column, and the eluent was CH 2 Cl 2 . Collect CH 2 Cl 2 The eluate was drained by a rotary evaporator, added ether and stirred until crystallization, and drained to obtain 0.782 g of the product. An appropriate amount of the...
Embodiment 2
[0076] Embodiment 2, antifreeze peptide composite prescription, when composed of antifreeze peptide, glycerin, mannitol, hydroxypropyl methylcellulose and sterile multiple distilled water, can be used for the protection of skin under low temperature environment.
[0077]
[0078] First soak the hydroxypropyl methylcellulose in the above formula in sterile multiple distilled water, and then add the antifreeze peptide and mannitol pre-dissolved in sterile multiple distilled water after it is completely swelled, then add glycerin, stir well That's it.
Embodiment 3
[0079] Embodiment 3, antifreeze peptide compound prescription, by antifreeze peptide, carbomer, glycerin, ethylparaben, triethanolamine appropriate amount (adjust pH to 6~9), sterile multiply distilled water to make hydrogel , can be used for protection of exposed skin in low temperature environment.
[0080]
[0081] Dissolve the carbomer resin in water first, and after it is completely swollen, add glycerin and mix evenly, or pass through a colloid mill, and then add triethanolamine to neutralize until the pH is 6-9 to obtain a transparent gel. When adding triethanolamine, minimize the generation of bubbles. Then add the antifreeze peptide aqueous solution into the above-mentioned gel, stir evenly and divide into packages. This gel is water-soluble, transparent and beautiful in appearance, and has a special delicate and smooth feeling when applied to the skin. It has an excellent coupling effect with the skin and can prevent the skin from frostbite caused by the low temp...
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