Compound Intumescent Flame Retardant for Rigid Polyurethane Foam
An intumescent flame retardant and matching technology, applied in the field of flame retardant, can solve problems such as the influence of the mechanical properties of the matrix, and achieve the effects of improving mechanical properties, improving thermal stability and simple preparation process
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Embodiment 1
[0022] The preparation of phosphorus-nitrogen expansion type polyol (PDTM) of the present invention:
[0023] Disperse 0.1 mol of pentaerythritol phosphorus oxychloride in acetone / water and place it in a three-necked flask, add 0.15 mol of aminotrimethylolmethane and 0.2 mol of triethylamine, react at room temperature for 2 hours (or 3 hours, or 4 hours), and then react at 40°C Reaction for 1h (or 1.5h, or 2h); vacuum rotary evaporation to remove the solvent and acid-binding agent to obtain a white solid, which was washed and purified to obtain the target product PDTM with a yield of over 90%.
Embodiment 2 to 6
[0025] The preparation of flame-retardant rigid polyurethane foam by compounding phosphorus-nitrogen expandable polyol (PDTM) and expandable graphite (EG) according to the present invention will be further illustrated by specific examples below. Polyether 4110 polyol (JH-4110), expandable polyol flame retardant (PDTM), expandable graphite (EG), dibutyltin dilaurate (DBTDL), triethanolamine (THA), foam stabilizer silicone oil (SD-201), water and other reasonable formula mixing (isocyanate index R = 1.05 ~ 1.1), rapid stirring for 3 minutes, then add polymethylene polyphenyl isocyanate (PM-200) into the mixing system, rapid stirring After 20 seconds, add it to the mold, control the volume and shape it, and then cure it in an oven at 70°C for 12 hours to get a flame-retardant rigid polyurethane foam, and the density of the obtained sample is basically controlled at 50kg / m 3 about. Test and compare the LOI test values under the condition of adding different components and conte...
Embodiment 7 to 11
[0029] Polyether 4110 polyol (JH-4110), expandable polyol flame retardant (PDTM), expandable graphite (EG), dibutyltin silicate (DBTDL), tertiary amine catalyst A33, foam stabilizer silicone oil ( AK8803), water and physical foaming agent (HCFC-141b) and other reasonable formulations (isocyanate index R = 1.05 ~ 1.1), rapid stirring for 3 minutes, and then polymethylene polyphenyl isocyanate (PM-200) was added to the In the mixing system, stir quickly for 20s, transfer to the mold, control the volume for molding, and cure in an oven at 70°C for 12 hours after molding to obtain a flame-retardant rigid polyurethane foam, and the density of the obtained sample is basically controlled at 50kg / m 3 about. Test and compare the LOI test values under the condition of adding different components and contents of flame retardants. Among them, Example 7 is used as a comparison of non-flame retardant RPUF in this group of formulations. The specific data results are shown in Table 2. It s...
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