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Fe-based mercury remover and preparation method thereof

An iron-based mercury removal agent and additive technology, which is applied in the direction of catalyst activation/preparation, chemical instruments and methods, physical/chemical process catalysts, etc., can solve the problems of dangerous production process, high cost, and difficult active components, and achieve The effect of safe preparation process, low product cost and easy availability of raw materials

Inactive Publication Date: 2017-02-08
XIAN SUNWARD AEROSPACE MATERIAL CO LTD
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0004] At present, the metal sulfide-type mercury removal agents in the prior art mainly use copper sulfide as the main active component, but the use of copper as the active metal component for mercury removal is relatively expensive, resulting in heavy burdens on related companies, and The vulcanization method commonly used in the preparation process is gas-phase vulcanization, which requires the use of sulfur-containing gases such as hydrogen sulfide for vulcanization. The production process is relatively dangerous, the tail gas is difficult to handle, and the active components are difficult to vulcanize completely. These shortcomings restrict the use of metal sulfide mercury removal agents. develop

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0025] Weigh 100 g of sodium sulfide nonahydrate and dissolve it in 3800 mL of water, and cool the solution to -12 o C; Another 112 g of ferric nitrate nonahydrate was dissolved in 500 mL of water, then the ferric nitrate solution was added to the sodium sulfide solution, and the reaction temperature was controlled to be -10 o C, after the reaction is completed, the resulting product is filtered and washed, and then 122 g of pseudo-boehmite and 1.5 g of CMC are added to mix and grind and extruded, and then dried in a vacuum oven at 20 o Dry at C for 60 h to obtain the finished mercury removal agent, which contains 19% of the active component iron sulfide, 80% of the carrier pseudo-boehmite, and 1% of the additive CMC.

Embodiment 2

[0027] Weigh 113.5 g of sodium sulfide nonahydrate and dissolve it in 500 mL of water, and cool the solution to 10 o C; Another 75.6g ferric sulfate is slowly added to the sodium sulfide solution, and the reaction temperature is controlled to be 15 o C, after the reaction is completed, the resulting product is filtered and washed, and then 51.5 g of α-aluminum hydroxide and 2.5 g of safflower powder are added, mixed and rolled, then extruded, and dried in a vacuum oven at 20 o Dry at C for 60 hours to obtain the finished mercury removal agent, which contains 35% of the active component iron sulfide, 62% of the carrier α-aluminum hydroxide, and 3% of the additive scallop powder.

Embodiment 3

[0029] Weigh 200 g of ammonium sulfide solution, and cool the solution to 20 o C; Take another 95.5g of ferric chloride hexahydrate and dissolve it in 1000 mL of water, then add the ferric sulfate solution into the ammonium sulfide solution, and control the reaction temperature to be 25 o C, after the reaction is completed, the resulting product is filtered and washed, and then 33 g of molecular sieve powder and 3.7 g of maltodextrin are added, mixed and rolled, and extruded, and dried in a vacuum oven at 30 o Dry at C for 40 hours to obtain the finished mercury removal agent, which contains 50% of the active component iron sulfide, 45% of the carrier molecular sieve, and 5% of the additive maltodextrin.

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PUM

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Abstract

The invention belongs to the technical field of a mercury remover, and more specifically relates to a Fe-based mercury remover and a preparation method thereof. The mercury remover comprises an active component, a carrier and an auxiliary agent, the active component is ferric sulfide, the mass parts of the active component is 19-65%, the mass parts of the carrier is 30-80%, and the mass parts of the auxiliary agent is 1-5%. The ferric sulfide prepared by a deposition technology has high mercury removing capability, the mercury volume can reach 40% or more, the addition of the carrier can guarantee high intensity of the products in a usage process; a band extrusion technology is employed for direct moulding and de-watering to obtain the product mercury remover, gas phase sulfuration is not required, the preparation process is safe; iron is taken as an active metal component for removing mercury, the raw materials are easily acquired, the production cost is low, and the Fe-based mercury remover can promote the development of the metal sulfide mercury remover.

Description

technical field [0001] The invention belongs to the technical field of mercury removal agents, and in particular relates to an iron-based mercury removal agent and a preparation method thereof. Background technique [0002] Mercury is highly volatile, highly toxic and corrosive, and widely exists in coal-burning flue gas, natural gas, natural gas condensate, naphtha and distillate oil. In the industrial production process, mercury is seriously harmful and will Corrosion and perforation of the aluminum heat exchanger, poisoning of the downstream catalyst, and reduction of catalyst life. In addition, mercury has serious biological toxicity. After mercury is absorbed in the body, it will form highly toxic methylmercury, which will combine with the sulfhydryl group of biological enzymes, thereby destroying the activity of enzymes. Methylmercury entering the brain will cause brain atrophy , Invasion of nerve cells, and mercury is accumulative in organisms, and mercury will enter...

Claims

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Application Information

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IPC IPC(8): B01J31/28
CPCB01J31/28B01J37/32
Inventor 许龙龙贺强彭东冯毅敏李平利卫冰孙未勤
Owner XIAN SUNWARD AEROSPACE MATERIAL CO LTD