Diacerein crystal I and preparation method and application thereof
A kind of technology of diacerein and crystal form, applied in the field of diacerein crystal I and preparation thereof, can solve problems such as low absorption, low solubility of diacerein, low bioavailability, etc., achieve simple process, easy industrial Operation, good solubility
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Embodiment 1
[0034] Add diacerein (Hu Mengqi et al., A new method for the synthesis of diacerein, China Journal of Pharmaceutical Industry, 2017, 48 (9): 1270-1273) 1g, N, N-dimethyl Acetamide 6ml, heated at 70°C for 15min with stirring. Remove the heat, cool the feed solution to 250°C within 10 minutes in an ice-water bath at 0°C, keep it warm for 3 hours to crystallize; then filter with suction, rinse the filter cake with absolute ethanol, and dry under reduced pressure at 80°C to obtain diacerein crystals I 0.98g, yield 98%, purity 99.5%.
[0035] The 2θ of the X-ray powder diffraction pattern of the diacerein crystal I obtained above has characteristic absorption peaks at 6.5°, 11.0°, 13.5°, 21.1°, 23.4°, and 28.2°, and the error range of the 2θ value is ±0.2 °, X-ray powder diffraction pattern see figure 1 .
[0036] The diacerein crystal I obtained above has an endothermic peak at 249.2°C and a maximum endothermic peak at 252.5°C using DSC characterization. The crystal has a relat...
Embodiment 2
[0038] Add diacerein (Hu Mengqi et al., A new method for the synthesis of diacerein, China Journal of Pharmaceutical Industry, 2017, 48 (9): 1270-1273) 1g, N, N-dimethyl Acetamide 10ml, stirred and heated at 90°C for 15min. The heating was removed, and the feed solution was cooled to 25°C in an ice-water bath at 0°C within 10 minutes, and left to stand for crystallization for 1h. Suction filtration, rinse the filter cake with absolute ethanol, and dry under reduced pressure at 80°C to obtain 0.97 g of Diacerein Form I, with a yield of 97% and a purity of 99.5%.
[0039]The 2θ of the X-ray powder diffraction pattern of the diacerein crystal I obtained above has characteristic absorption peaks at 6.5°, 11.0°, 13.5°, 21.1°, 23.4°, and 28.2°, and the error range of the 2θ value is ±0.2 °, X-ray powder diffraction pattern see image 3 .
[0040] Referring to the method recorded in the article "Diacerein intervenes in the expression of connective tissue growth factor in cultured ...
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