Graphene modified sodium phosphate dibasic dodecahydrate hydrated phase change heat storage material and preparation method thereof
A hydration technology of disodium hydrogen phosphate dodecahydrate and disodium hydrogen phosphate, which is applied in the field of graphene-modified disodium hydrogen phosphate dodecahydrate hydrated phase-change heat storage materials and its preparation, can solve the problem of low heat storage efficiency and easy Avoid problems such as agglomeration and heat storage density reduction, and achieve the effect of avoiding phase separation, improving latent heat of phase change, and large value of latent heat of phase change
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[0030] The invention provides a method for preparing a graphene-modified disodium hydrogen phosphate dodecahydrate hydrated phase-change thermal storage material, comprising the following steps:
[0031] 1) mixing and refining disodium hydrogen phosphate dodecahydrate, graphene and nucleating agent into powder, and melting the powder to obtain graphene-modified disodium hydrogen phosphate dodecahydrate;
[0032] 2) Melt and mix graphene-modified disodium hydrogen phosphate dodecahydrate, thickener and anti-caking agent to obtain a gel-like mixture, which is the graphene-modified disodium hydrogen phosphate dodecahydrate hydrated phase change heat storage material .
[0033] In the present invention, the mixing speed in step 1) is 100-150r / min, and the mixing time is 20-30min; preferably, the mixing speed is 120-140r / min, and the mixing time is 22-28min; Further preferably, the mixing speed is 130r / min, and the mixing time is 25min.
[0034] In the present invention, the part...
Embodiment 1
[0042] 1) Mix 95 parts of disodium hydrogen phosphate dodecahydrate, 3 parts of graphene and 2 parts of sodium acetate trihydrate, and grind the mixture into a powder with a particle size of 100 μm, and place the powder in a container at 60 ° C under water bath conditions Heat for 30 minutes until the powder is completely melted, stir evenly, seal and cool to room temperature to obtain graphene-modified disodium hydrogen phosphate dodecahydrate;
[0043] 2) Heat the modified disodium hydrogen phosphate dodecahydrate obtained in the previous step, 1 part of sodium carboxymethyl cellulose, and 2 parts of activated tricalcium phosphate in a water bath at 90°C for 30 minutes until the mixture is completely melted and stirred evenly , the obtained colloidal mixture is the graphene-modified disodium hydrogen phosphate dodecahydrate hydrated phase change heat storage material.
Embodiment 2
[0045] 1) Mix 96 parts of disodium hydrogen phosphate dodecahydrate, 2 parts of graphene and 2 parts of disodium hydrogen phosphate, and grind the mixture into a powder with a particle size of 110 μm, put the powder in a container at 55°C under water bath conditions Heating for 40 minutes until the powder is completely melted, stirring evenly, sealing and cooling to room temperature to obtain graphene-modified disodium hydrogen phosphate dodecahydrate;
[0046] 2) Heat the modified disodium hydrogen phosphate dodecahydrate obtained in the previous step with 2 parts of polyvinyl alcohol and 0.5 part of calcium carbonate in a water bath at 85°C for 50 minutes until the mixture is completely melted and stirred evenly to obtain a colloidal The mixture is the graphene-modified disodium hydrogen phosphate dodecahydrate hydrated phase-change thermal storage material.
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