Method for improving electron transfer efficiency of flora in situ

A technology of electron transfer and efficiency, applied in chemical instruments and methods, water/sludge/sewage treatment, biological water/sewage treatment, etc., can solve the problems of accelerating electroactive microorganisms, low current utilization rate, complex treatment steps, etc. Achieve the effect of improving transfer efficiency, improving current utilization efficiency, and reducing tedious operation steps

Pending Publication Date: 2022-08-02
UNIV OF JINAN
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Problems solved by technology

[0002] The three-dimensional electrocatalytic biofilm system has been applied to treat wastewater such as organic and heavy metal ions, but the current three-dimensional electrocatalytic biofilm system still has problems such as low current utilization rate and high energy consumption. An important factor for the efficient operation of the membrane system
Sewage and wastewater containing metal ions are currently mainly used to remove and recover metal ions from sewage through various treatment technologies, and the treatment steps are complicated.
Studies have shown that some microorganisms such as G.sulfurreducens PCA, Shewanella sp., etc. can mineralize heavy metal ions to form sediments or nanoparticles, which can accelerate the formation of electroactive microorganisms to form electroactive biofilms, but the use of them in sewage treatment is still relatively limited. few

Method used

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Embodiment example 1

[0028] 1) To build a three-dimensional electro-biofilm system, the effective volume of the reactor is 10L, the cathode is stainless steel, the anode is a graphite rod, and the particle electrode is activated carbon particles with a particle size of 3~5mm, and the usage amount is 250g / L. The pH value of the control reactor was 7.0±0.2, the temperature was 25±2°C, and a constant potential of 2V was applied. Organic wastewater with an initial concentration of tetracycline of 5.0 mg / L and a COD concentration of 1200 mg / L was continuously fed, and the influent flow was 30 mL / min. After 12 hours of suffocating exposure, the water supply was stopped to discharge the sewage from the reactor, and the water was re-injected for suffocating exposure, and the water was repeatedly changed for suffocating exposure for two days. The concentration of tetracycline in the influent is 1 mg•L -1 The gradient of / d was gradually increased to be constant at the concentration of 20 mg / L. Co-culture...

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Abstract

The invention provides a method for improving the electron transfer efficiency of a flora in situ, which is suitable for wastewater treatment of a three-dimensional electro-catalysis biological membrane system. The method comprises the following steps: firstly, constructing a three-dimensional electro-catalysis biological membrane system to culture an electro-active microbial membrane with target pollutant degradation capacity, then periodically regulating and controlling the electric field intensity to selectively enrich the electro-active microbial membrane, and finally, introducing low-concentration metal ion wastewater according to a certain flow ratio and controlling the current density. And nano-particles are synthesized in situ inside or on the surfaces of the microorganisms on the main electrode and the particle electrode. The biomineralization synthesized nanoparticles are tightly combined with cell membranes and periplasmic space, idle and dead electron conduits are connected, the electron transfer efficiency between organisms and electron acceptors and between organisms and non-biological interfaces is improved, the electron transfer process is improved, the current utilization efficiency of a three-dimensional electro-catalysis biological membrane system is further improved, and the service life of the three-dimensional electro-catalysis biological membrane system is prolonged. The treatment energy consumption is reduced; and pollutants can be efficiently degraded.

Description

technical field [0001] The invention belongs to the field of water treatment and provides an in-situ method for improving the electron transfer efficiency of bacterial groups, which is suitable for wastewater treatment by a three-dimensional electrocatalytic biofilm system. Background technique [0002] The three-dimensional electrocatalytic biofilm system has been applied to the treatment of organic and heavy metal ions and other wastewater. However, the current three-dimensional electrocatalytic biofilm system still has problems such as low current utilization rate and high energy consumption. An important factor for the efficient operation of a membrane system. [0003] Electroactive microorganisms transfer electrons generated by intracellular oxidative electron donors to extracellular electron acceptors or take up electrons through specific respiratory chains, reducing the power of cathode electrodes to save energy or maintain their metabolic activity. These processes ar...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): C02F3/00C02F101/20C02F101/30C02F101/34C02F101/38
CPCC02F3/005C02F2101/30C02F2101/20C02F2101/203C02F2101/38C02F2101/34Y02W10/10
Inventor 黄清铃李子晨冯岩盛辉辉
Owner UNIV OF JINAN
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