High-temperature resistant peelable water-based silica sol polyurethane microcapsule emulsion and preparation method thereof
A technology of polyurethane microcapsules and water-based silicon, applied in the direction of polyurea/polyurethane coatings, coatings, etc., can solve the problem that the temperature resistance cannot be taken into account, and achieve the effects of low cost, excellent temperature resistance and simple process flow
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Embodiment 1
[0028] The components and parts by weight of the high temperature-resistant peelable water-based silica sol polyurethane microcapsule emulsion of this embodiment are shown in Table 1. Its preparation method comprises the following steps:
[0029] (1) 26 parts of polybutylene adipate diol with a number average molecular weight of 2000 were vacuum dehydrated at 130°C for 1.5h, and then placed in a three-necked flask equipped with a stirrer, a reflux condenser, and a thermometer , lower the temperature to 50°C, add 22 parts of diphenylmethane diisocyanate (MDI), and control the temperature at 75°C for 2.5 hours;
[0030] (2) Add 4 parts of dimethylolpropionic acid (DMPA) to react for 2 hours, add 2.5 parts of 1,4 butanediol to react for 2 hours;
[0031] (3) Lower the temperature to 40°C, add 4 parts of neutralizing agent triethylamine (TEA) to neutralize for 1 hour, then discharge the material, add to the aqueous silica sol solution diluted with 15 parts of silica sol with 180 ...
Embodiment 2
[0034] The components and parts by weight of the high temperature-resistant peelable water-based silica sol polyurethane microcapsule emulsion of this embodiment are shown in Table 1. Its preparation method comprises the following steps:
[0035] (1) 38 parts of polyneopentyl glycol adipate diol with a number average molecular weight of 3000 were vacuum dehydrated at 120°C for 1 hour, and then placed in a three-necked flask equipped with a stirrer, a reflux condenser, and a thermometer , then lower the temperature to 60°C, add a mixture of 34 parts of toluene diisocyanate (TDI), control the temperature at 80°C, and copolymerize for 3 hours;
[0036] (2) Add 9 parts of dimethylolbutyric acid for hydrophilic chain extension reaction, the reaction time is 1.5h, then add 7 parts of neopentyl glycol for 3h;
[0037] (3) Lower the temperature to 40°C, then add 9 parts of dimethylethanolamine to neutralize for 0.5h, then discharge, add to the aqueous silica sol solution diluted with...
Embodiment 3
[0040] The components and parts by weight of the high temperature-resistant peelable water-based silica sol polyurethane microcapsule emulsion of this embodiment are shown in Table 1. Its preparation method comprises the following steps:
[0041] (1) Vacuum dehydrate 32 parts of polycaprolactone polyol with a number average molecular weight of 1500 at 125°C for 1 hour, then place it in a three-necked flask equipped with a stirrer, reflux condenser, and thermometer, and then cool it down to 55°C ℃, add 26 parts of isophorone diisocyanate (IPDI), control the temperature at 85 ℃, and copolymerize for 2.5 hours;
[0042] (2) Add 6.5 parts of dimethylolbutyric acid for chain extension reaction, the reaction time is 1h, add 4 parts of ethylene glycol to react for 2.5h;
[0043] (3) Lower the temperature to 45°C, then add 6.5 parts of triethanolamine to neutralize for 1 hour, then discharge, add to the aqueous silica sol solution diluted with 30 parts of silica sol with 250 parts of...
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