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Preparation method and application of formed magnetism modified cellulose

A technology of cellulose and carboxymethyl cellulose, which is applied in the field of polymer chemical materials, can solve problems such as poor pore structure and poor hydraulic performance, and achieve the effect of simple and easy preparation process and low raw material cost

Active Publication Date: 2014-05-21
FUJIAN UNIV OF TECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0004] Publication No. CN101274985, the Chinese patent titled "a magnetic cellulose microsphere and its preparation method and application" discloses that iron-cobalt-nickel superparamagnetic inorganic particles are used as magnetic fluid, and alkali / urea or sulfur The aqueous solution of urea is used as the solvent, and the magnetic cellulose solution is prepared by the direct embedding method, and then the magnetic cellulose microspheres with high magnetic response are prepared by the sol-gel phase inversion method at room temperature; this scheme uses iron-cobalt-nickel inorganic particles as the magnetic fluid , the prepared product is in powder form, which has disadvantages such as poor hydraulic properties and poor pore structure.

Method used

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preparation example Construction

[0013] The preparation method of the molding magnetically modified cellulose of the present invention specifically comprises the following steps:

[0014] Step (1), preparation of modified cellulose: add 90% ethanol to sodium carboxymethyl cellulose until it becomes viscous, and adjust the pH to 1-2, stir for 1 hour, let it stand for 4 hours, and then filter it with suction. After suction filtration, the substances on the filter paper are washed with water and ethanol in sequence, and then dried at 80°C to a constant weight to obtain carboxymethyl cellulose for later use; take diethylenetriamine and the obtained carboxymethyl cellulose at a molar ratio of 4:1 Base cellulose is reacted to obtain modified cellulose, and the reaction temperature is 100°C and the reaction time is 6h;

[0015] Step (2), preparation of shaped magnetically modified cellulose: Fe prepared by co-precipitation method 3 o 4 As magnetic particles, take the magnetic particles for initial ultrasonic treat...

Embodiment 1

[0021] Cd 2+ Preparation of contaminated soil: The soil for the test was taken from the farmland in the suburbs of Shangjie Town, Minhou County, all of which are farmland soil in the plow layer (0-20cm topsoil), and was naturally air-dried indoors to constant weight to remove impurities, and passed through a 20-mesh sieve after grinding , for standby; known through measurement, the pH value of the initial test soil is 4.81, and the cadmium ion concentration is

[0022] 1.9mg / kg, moisture content 18%; take the soil that has been air-dried to constant weight and ground through a 20-mesh sieve, which is the spare soil, and add a cadmium chloride solution with a concentration of 2mol / L to the spare soil at room temperature And stir for 6 hours to ensure that the soil and the configured heavy metal solution, i.e. the cadmium chloride solution, are fully mixed. After the stirring is complete, take it out and place it in a larger tray to air-dry naturally, and stabilize it for 2 week...

Embodiment 2

[0025] Cd 2+ Preparation of contaminated soil: The soil for testing was taken from the farmland of Datian County, Sanming City, all of which were cultivated farmland soil (0-20cm topsoil), and was naturally air-dried indoors to constant weight to remove impurities, and then ground and passed through a 20-mesh sieve for later use; It is known through measurement that the pH value of the initial test soil is 3.5, the concentration of cadmium ions is 2.5 mg / kg, and the moisture content is 20%; the soil that has been air-dried to constant weight and ground through a 20-mesh sieve is the soil for subsequent use. Add the 2.5mol / L cadmium chloride solution to the spare soil at room temperature and stir for 6 hours to ensure that the soil and the prepared heavy metal solution, that is, the cadmium chloride solution, are fully mixed. After the stirring is complete, take it out and place it in a larger tray Naturally air-dried, stabilized and balanced for 2 weeks, obtained the Cd of thi...

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PUM

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Abstract

The invention provides a preparation method a formed magnetism modified cellulose. The preparation method comprises the step that with inorganic magnetic particles, namely, ferroferric oxide, as magnetic flow, and with cellulose additive, namely, sodium carboxymethylcellulose, as raw material, modifying, and forming, so as to prepare the formed magnetism modified cellulose; the whole preparation process is simple and practicable, and the raw materials are cheap, therefore the preparation method is suitable for large-scale promotion; furthermore, the prepared formed magnetism modified cellulose has excellent restoring effect to heavy metal Cd pollution in soil.

Description

【Technical field】 [0001] The invention belongs to the field of polymer chemical materials, and in particular relates to a preparation method and application of shaped magnetically modified cellulose. 【Background technique】 [0002] Cellulose is the most abundant natural polymer compound in nature, which has the advantages of easy biodegradation and regeneration. Cellulose and its derivatives contain a variety of functional groups, so they exhibit strong adsorption capacity for heavy metals and have selective properties. However, the current modified cellulose mainly exists in the form of powder, granular and fibrous, which has poor hydraulic properties and poor pore structure. These shortcomings limit the application field of modified cellulose. Magnetic polymers are a new product that combines inorganic magnetic particles / polymers, which overcomes their simple shortcomings, and under the synergistic effect, obtains better characteristics than polymers and inorganic particl...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): B01J20/24B01J20/28B01J20/30C08B15/06B09C1/00
Inventor 刘心中孙佳黄永捷
Owner FUJIAN UNIV OF TECH