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Cyclohexanone-melamine-formaldehyde polycondensation resin and preparation method thereof

A technology of co-condensation resin and melamine, which is applied in the field of coating/ink additives, can solve the problems of weak anti-yellowing performance, low softening point, and poor anti-powdering ability, and achieve good solvent compatibility and high resin yield , the effect of improving performance

Active Publication Date: 2016-05-25
YUEYANG INTECH SYNTHETIC MATERIALS
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0005] Keto-aldehyde resin is a thermoplastic resin, which has the disadvantages of low softening point, poor anti-powdering ability, and weak anti-yellowing performance.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0033] Catalyst: 30 parts by mass of sodium hydroxide and 70 parts by mass of deionized water are made into an aqueous catalyst solution for future use.

[0034] Add 126kg of melamine and 500kg of 37% industrial formaldehyde solution into the reaction kettle, adjust the pH value to 9 with the catalyst aqueous solution, heat up to 80°C, keep the temperature for 3 hours, detect and adjust the pH value to 10 with the catalyst aqueous solution; join the industrial 980kg of cyclohexanone and 560kg of 37% industrial formaldehyde solution adjusted to pH 10 in advance with catalyst aqueous solution, stirred, kept reacting at 90°C for 5h, added deionized water, and washed the resin 6 times at 80°C. After washing for the first time, vacuum the upper layer of water; heat up and evaporate, when the temperature reaches 110°C, turn on the vacuum pump, gradually evacuate to -0.098Mpa, gradually raise the temperature to 150°C, keep the temperature and vacuum for 1 hour, stop Stir, feed nitrog...

Embodiment 2

[0036] Catalyst: 20 parts by mass of 80% potassium hydroxide and 80 parts by mass of deionized water are made into an aqueous catalyst solution for future use.

[0037] Add 100kg of melamine and 300kg of 37% industrial formaldehyde solution into the reaction kettle, adjust the pH value to 11 with an aqueous catalyst solution, heat up to 80°C, keep the temperature for 1 hour, detect and adjust the pH value to 11 with an aqueous catalyst solution; join the industrial Cyclohexanone kg and 1000 kg of 37% industrial formaldehyde solution adjusted to pH 10 in advance with the catalyst aqueous solution, stirred, kept reacting at 100°C for 2h, added deionized water, and washed the resin 4 times at 90°C, each After washing for the first time, use vacuum to absorb the upper layer of water; heat up and evaporate, when the temperature reaches 110°C, turn on the vacuum pump, gradually evacuate to -0.098Mpa, gradually raise the temperature to 150°C, and keep the temperature and vacuum for 1 ...

Embodiment 3

[0039] Catalyst: 30 parts by mass of sodium hydroxide, 10 parts by mass of 80% potassium hydroxide, and 60 parts by mass of deionized water, made into an aqueous catalyst solution for future use.

[0040] Add 150kg of melamine and 400kg of 37% industrial formaldehyde solution into the reaction kettle, adjust the pH value to 10 with an aqueous catalyst solution, heat up to 70°C, keep the temperature for 2 hours, detect and adjust the pH value to 12 with an aqueous catalyst solution; join the industrial 1020kg of cyclohexanone and 1060kg of 37% industrial formaldehyde solution whose pH value was adjusted to 10 with a catalyst aqueous solution in advance, stirred, kept reacting at 90°C for 4h, added deionized water, and washed the resin 5 times at 90°C. After washing for the first time, use vacuum to absorb the upper layer of water; heat up and evaporate, when the temperature reaches 110°C, turn on the vacuum pump, gradually evacuate to -0.098Mpa, gradually raise the temperature t...

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Abstract

The invention discloses a cyclohexanone-melamine-formaldehyde co-polycondensation resin, which is prepared by reacting melamine with formaldehyde under the action of a catalyst, and then adding cyclohexanone for co-polycondensation, and the catalyst is an alkali metal hydrogen Oxide, or more than one alkali metal hydroxide mixture, its preparation method includes: adding melamine and formaldehyde into the reactor, adding a catalyst to adjust the pH value to 10-12, stirring and raising the temperature to 60-80 ° C, When the pH is 10-12, keep the temperature for 0.5-2h; add cyclohexanone, stir and react at 90-100°C for 2-6h; add deionized water, wash with water for 2-6 times at a temperature of 80-90°C; vacuum After evaporation, cyclohexanone-melamine-formaldehyde polycondensation resin is obtained. The resin prepared by the present invention has good compatibility with solvent and resin, has higher glass transition temperature and softening point than cyclohexanone-formaldehyde resin, and better anti-yellowing property, and is a new type of coating / ink auxiliary agent resin.

Description

technical field [0001] The invention relates to the technical field of paint / ink additives, more specifically, to a cyclohexanone-melamine-formaldehyde co-condensation resin used as a paint / ink additive and a preparation method thereof. Background technique [0002] Keto-formaldehyde resin is a kind of paint / ink additive, which is a kind of resin formed by condensing ketones and formaldehyde. Currently the most widely used is cyclohexanone-formaldehyde resin. It is a polycondensation of cyclohexanone and formaldehyde under the catalysis of alkali, which contains carbonyl and the terminal group is hydroxyl. This kind of resin has good compatibility with other resins, and when it is used in coatings and inks, it can effectively improve its gloss, adhesion, hardness and other properties. [0003] For example, the Chinese patent CN1837253A "preparation method of cyclohexanone-formaldehyde resin" applied by Zhang Yifu, the Chinese patent CN1281867A "a kind of manufacturing meth...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C08G6/02C08G12/40C08G12/32
Inventor 张一甫黄劲易新亮张建华刘行军
Owner YUEYANG INTECH SYNTHETIC MATERIALS