A kind of high-toughness two-dimensional ultra-thin titanium dioxide modified pp nanocomposite material and preparation method thereof
A nanocomposite material, titanium dioxide technology, applied in the field of two-dimensional ultra-thin TiO2 modified PP nanocomposite material and its preparation, can solve problems such as hardening, easy aging, and long-term use limitation
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[0033] The invention provides a method for preparing a high-toughness two-dimensional ultra-thin titanium dioxide modified PP nanocomposite material, comprising
[0034] Step 1: Preparation of two-dimensional ultrathin nano-TiO 2
[0035] Under the protection of nitrogen, add titanium tetrachloride to ethylene glycol, heat to reflux, and then add water to react. After the reaction, cool down to room temperature, centrifuge and wash to obtain two-dimensional ultra-thin nano-TiO 2 ; The reaction time is preferably 30min-5h; more preferably 2-4h, the volume ratio of ethylene glycol and titanium tetrachloride is preferably (5-100): 1, more preferably (5-6) : 1, the volume ratio of titanium tetrachloride to water is preferably (1-4): 1, more preferably (1-1.25): 1; the ethylene glycol is used as a directing agent;
[0036] Step 2: Modified two-dimensional ultrathin nano-TiO 2
[0037] Surfactant and two-dimensional ultrathin nano-TiO 2 reaction to obtain modified two-dimension...
Embodiment 1
[0044] Under the protection of nitrogen, add 0.5L titanium tetrachloride to 3.0L ethylene glycol, heat to reflux, add 0.5L water to react with titanium tetrachloride, react for 2.0h, cool down to room temperature, and perform centrifugation and washing. Two-dimensional ultrathin nano-TiO 2 .
[0045] two-dimensional ultrathin nano-TiO 2 Reversely disperse in a mixed solution of water and ethanol (the volume ratio of water and ethanol is 9:1), super-disperse for 50min, then add surfactant KH550, react at 70°C for 4h, after cooling, centrifuge at 5000r / min, and dry at 100°C Overnight, the addition of the surfactant is two-dimensional ultra-thin nano-TiO 2 2.5% of the mass; modified two-dimensional ultrathin nano-TiO 2 -M (thickness 20nm, aspect ratio 15).
[0046] The PP material and the modified two-dimensional ultrathin nano-TiO 2 -M drying, the drying temperature is 100°C, and the drying time is 6 hours, which can improve the processing performance of the material; then ...
Embodiment 2
[0050] Under the protection of nitrogen, add 0.5L titanium tetrachloride to 3.0L ethylene glycol, heat to reflux, add 0.5L water to react with titanium tetrachloride, react for 2.0h, cool down to room temperature, and perform centrifugation and washing. Two-dimensional ultrathin nano-TiO 2 .
[0051] two-dimensional ultrathin nano-TiO 2 Reversely disperse in a mixed solution of water and ethanol (the volume ratio of water and ethanol is 9:1), super-disperse for 50min, then add surfactant KH550, react at 70°C for 4h, after cooling, centrifuge at 5000r / min, and dry at 100°C Overnight, the addition of the surfactant is two-dimensional ultra-thin nano-TiO 2 2.5% of the mass; modified two-dimensional ultrathin nano-TiO 2 -M (thickness 20nm, aspect ratio 15).
[0052] The PP material and the modified two-dimensional ultrathin nano-TiO 2 -M drying, the drying temperature is 100°C, and the drying time is 6 hours, which can improve the processing performance of the material; then ...
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