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Ultrafine zirconia/sic composite long fiber and its preparation method and application

A long fiber and reaction technology, applied in the field of ultrafine ZrO2/SiC composite long fiber and its preparation, can solve the problems of poor oxidation resistance, cannot exceed 500 ℃, mismatched thermophysical properties, etc., and achieves simple process and comprehensive performance. Good results

Active Publication Date: 2022-03-04
JIANGXI JIAJIEXINDA NEW MATERIAL TECH CO LTD
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0002] Carbon / carbon (C / C) composites are common ablation-resistant materials, and their temperature resistance can exceed 2000°C in an inert atmosphere. However, the fatal disadvantage of C / C composites is their poor oxidation resistance. The temperature cannot exceed 500°C. Preparation of ultra-high temperature resistant ceramic coating on the surface of C / C and doping the substrate can improve its ablation resistance and oxidation resistance, but the coating or doping will cause mismatching of thermophysical properties And other issues

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0015] Embodiment 1 proposes a kind of ultrafine ZrO 2 The preparation method of / SiC composite long fiber, comprises the steps:

[0016] (1) first drop glycerol and trimethylmonochlorosilane in dimethyldichlorosilane under stirring, then add reaction metal and xylene, then heat until the reaction metal melts into a liquid state and stir until The solution turns purple until the purple is no longer deep, then lower the temperature to room temperature, then cool and filter, wash with alcohol, dry and grind into powder; among them, dimethyldichlorosilane, glycerol and trimethylchlorosilane The mass ratio is 10:2:1; the reaction metal is 7% of the total mass of the reactants, and the xylene is 8% of the total volume of the reactants. The reactive metal is magnesium.

[0017] (2) Add the powder into the reaction device and fill it with protective gas, then heat it to 160°C and keep it warm for 5 hours, then add phenol and formaldehyde to obtain methylphenol; wherein, the volume r...

Embodiment 2

[0021] Embodiment 2 proposes a kind of ultrafine ZrO 2 The preparation method of / SiC composite long fiber, comprises the steps:

[0022] (1) first drop glycerol and trimethylmonochlorosilane in dimethyldichlorosilane under stirring, then add reaction metal and xylene, then heat until the reaction metal melts into a liquid state and stir until The solution turns purple until the purple is no longer deep, then lower the temperature to room temperature, then cool and filter, wash with alcohol, dry and grind into powder; among them, dimethyldichlorosilane, glycerol and trimethylchlorosilane The mass ratio is 10:2:1; the reaction metal is 13% of the total mass of the reactants, and xylene is 5% of the total volume of the reactants. The reactive metal is sodium.

[0023] (2) Add the powder into the reaction device and fill it with protective gas, then heat it to 220°C and keep it warm for 3 hours, then add phenol and formaldehyde to obtain methylphenol; wherein, the volume ratio o...

Embodiment 3

[0027] Embodiment 3 proposes a kind of ultrafine ZrO 2 The preparation method of / SiC composite long fiber, comprises the steps:

[0028] (1) first drop glycerol and trimethylmonochlorosilane in dimethyldichlorosilane under stirring, then add reaction metal and xylene, then heat until the reaction metal melts into a liquid state and stir until The solution turns purple until the purple is no longer deep, then lower the temperature to room temperature, then cool and filter, wash with alcohol, dry and grind into powder; among them, dimethyldichlorosilane, glycerol and trimethylchlorosilane The mass ratio is 10:2:1; the reaction metal is 10% of the total mass of the reactants, and xylene is 7% of the total volume of the reactants. The reactive metal is potassium.

[0029] (2) Add the powder into the reaction device and fill it with protective gas, then heat it to 190°C and keep it warm for 4 hours, then add phenol and formaldehyde to obtain methylphenol; wherein, the volume rati...

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Abstract

The present invention relates to a kind of ultrafine ZrO 2 / SiC composite long fiber and its preparation method and application, the method comprises the steps of: dripping glycerol and trimethylmonochlorosilane in dimethyldichlorosilane, then adding reaction metal and xylene, and then heating to The reaction metal melts into a liquid and turns purple, cools and filters, then dries and grinds into powder and heats, then adds phenol and formaldehyde to obtain methylphenol; dissolves the zirconium oxychloride hybrid solution in ethanol, adds Acetyl acetone to obtain a zirconium-containing complex, which is added to the methyl phenol to obtain the ZrC precursor polymer methyl phenol ethyl phthalate zirconone; adopt the melt spinning method to obtain ultrafine ZrO 2 / SiC composite long fiber. Ultrafine ZrO of the present invention 2 The raw materials used in the preparation of / SiC composite long fiber materials are easy to get and cheap, the process is simple, and the obtained ultrafine ZrO 2 / SiC composite long fiber material has good comprehensive performance and is suitable for manufacturing core components for aerospace heat protection.

Description

technical field [0001] The present invention relates to a kind of superfine ZrO 2 / SiC composite long fiber and its preparation method and application. Background technique [0002] Carbon / carbon (C / C) composites are common ablation-resistant materials, and their temperature resistance can exceed 2000°C in an inert atmosphere. However, the fatal disadvantage of C / C composites is their poor oxidation resistance. The temperature cannot exceed 500°C. Preparation of ultra-high temperature resistant ceramic coating on the surface of C / C and doping the substrate can improve its ablation resistance and oxidation resistance, but the coating or doping will cause mismatching of thermophysical properties And other issues. Contents of the invention [0003] An object of the present invention is to propose a kind of superfine ZrO with anti-oxidation and anti-fracture performance advantage 2 / SiC composite long fiber preparation method. [0004] A kind of ultrafine ZrO of the presen...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C04B35/622D01F9/10
CPCC04B35/62281C04B35/6225D01F9/10C04B2235/6567C04B2235/94C04B2235/96
Inventor 吴宝林侯振华
Owner JIANGXI JIAJIEXINDA NEW MATERIAL TECH CO LTD