Fluorine surfactant as well as preparation method and application thereof
A technology of fluorosurfactants and surfactants, applied in the field of fluorosurfactants and their preparation, can solve the problems of unstable small molecular substances, cumbersome preparation methods of copolymers, and incomplete removal of impurities, so as to reduce the droplet Effects of surface tension, ensuring stability, and simple synthesis method
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[0044] The present invention also provides a kind of preparation method of above-mentioned fluorosurfactant, comprises the following steps:
[0045] (1) Preparation of the intermediate: Dissolve the fluorine-containing polyether with the structure of formula III and the oxalyl chloride with the structure of formula IV in a solvent, and remove the solvent after heating for 6h to 12h to obtain the intermediate with the structure of formula V;
[0046]
[0047] (2) Synthesis of fluorosurfactant: add Tween 20 of formula VI structure and mixed solvent to the intermediate of formula V structure, heat and stir to obtain the compound of formula I structure;
[0048]
[0049] In the preparation method provided by the present invention, the fluorosurfactant can be directly reacted without using a catalyst, and what is prepared is a non-existing three-stage fluorosurfactant, the preparation method is simple, and the preparation process is simplified. route.
[0050] In a specific ...
Embodiment 1
[0062] A kind of fluorosurfactant, molecular formula is [C 3 f 7 O(C 3 f 6 O) n CO] m C 26 h 60-m o 10 , wherein, n=32-40, m=3, obtain by following preparation method:
[0063] Weigh 60g of fluorine-containing polyether and dissolve in 500mL of HFE7100, add 100mL of oxalyl chloride, heat to reflux and stir for 16h, and then remove the solvent under reduced pressure. Add 3.6g of Tween 20, 100mL of HFE7100, and 20mL of tetrahydrofuran, heat to reflux and stir for 24h, filter the reaction solution, add 100mL of absolute ethanol while stirring, remove the viscous material in the lower layer, and dry it in vacuo.
Embodiment 2
[0065] A kind of fluorosurfactant, molecular formula is [C 3 f 7 O(C 3 f 6 O) n CO] m C 26 h 60-m o 10 , wherein, n=32-40, m=2, obtain by following preparation method:
[0066] Weigh 60g of fluorine-containing polyether and dissolve in 500mL of HFE7100, add 100mL of oxalyl chloride, heat to reflux and stir for 16h, and then remove the solvent under reduced pressure. Add 5.4g of Tween 20, 100mL of HFE7100, 20mL of tetrahydrofuran, heat to reflux and stir for 24h, filter the reaction solution, add 100mL of absolute ethanol while stirring, remove the viscous material in the lower layer, and dry it in vacuo.
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