Antibacterial polyethylene material and preparation method thereof
A technology of polyethylene and hydroxypolyethylene, applied in botany equipment and methods, chemicals for biological control, biocides, etc., can solve the problems of easy discoloration, poor heat resistance, and low safety of antibacterial agents, and achieve Excellent water resistance, high antibacterial efficiency, and easy handling
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Embodiment 1
[0030] Preparation of polyethylene macromolecular chain transfer agent.
[0031] Add 3-benzylsulfanylthiocarbonylsulfanylpropionic acid (6.0mmol) and 20ml of anhydrous tetrahydrofuran THF in a 50mL branched flask, place the branched flask on the reactor, and raise the temperature of the reactor to 70 ℃, slowly drop SOCl 2 (6.0mmol), the dropwise addition was completed, and the reaction was continued for 2.5h. After the reaction was completed, the product was cooled to room temperature, and the SOCl was removed by distillation under reduced pressure. 2 and THF to give 3-benzylsulfanylthiocarbonylsulfanylpropionyl chloride.
[0032] N 2 Under protection, add single-terminal hydroxypolyethylene (1.0mmol) into a 50ml Schlenk bottle, add 30ml of anhydrous toluene, heat up to 60°C, after the single-terminal hydroxypolyethylene is completely dissolved, add 1ml of pyridine, stir for 30min, drop Add the above-mentioned 3-benzylsulfanylthiocarbonylsulfanylpropionyl chloride dissolved...
Embodiment 2
[0034] Preparation of antimicrobial polyethylene materials.
[0035] N 2 Under protection, polyethylene macromolecular chain transfer agent (0.1mmol), azobisisobutyronitrile (0.01mmol), 2-guanidino ethyl acrylate hydrochloride (5.0mmol) were added to a 25ml Schlenk bottle, and 5mL of dioxane, raise the temperature of the reactor to 70°C, react for 1h, put the product into liquid nitrogen to quench the reaction to stop the reaction, add the product dropwise to methanol / water to precipitate out, dissolve the precipitate 3 times continuously, filter, And washed with methanol, dried in vacuum at 45° C. to constant weight to obtain an antibacterial polyethylene material with a yield of 84.9%.
Embodiment 3
[0037] Preparation of antimicrobial polyethylene materials.
[0038] N 2 Under protection, polyethylene macromolecular chain transfer agent (0.1mmol), azobisisobutyronitrile (0.01mmol), 2-guanidino ethyl acrylate hydrochloride (5.0mmol) were added to a 25ml Schlenk bottle, and 5mL of dioxane, raise the temperature of the reactor to 70°C, react for 1.5h, put the product into liquid nitrogen to quench the reaction to stop, add the product dropwise to methanol / water to precipitate out, dissolve the precipitate 3 times continuously, filter , and washed with methanol, dried under vacuum at 45° C. to constant weight to obtain an antibacterial polyethylene material with a yield of 86.1%.
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