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Method for preparing ginseng saponin F2 by enzymatic hydrolysis of ginseng saponin Rb1

A technology of ginsenoside and enzymatic hydrolysis, applied in the direction of microorganism-based methods, biochemical equipment and methods, microorganisms, etc., can solve the problems of cumbersome separation and complex components of reaction products, and achieve low process cost and benefit large quantities The effect of mild preparation and reaction conditions

Inactive Publication Date: 2011-11-16
EAST CHINA UNIV OF SCI & TECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

The microbial fermentation method has strong specificity, mild conditions, and less environmental pollution, but has the disadvantages of complex components of the reaction product and cumbersome separation

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0014] Cultivate Fusarium ECU2042 in Chase's medium, medium composition: sucrose 30g / l, NaNO 3 3.0g / l, K 2 HPO 4 1.0g / l, KCl 0.5g / l, MgSO 4 ·7H 2 O 0.5g / l, FeSO 4 ·7H 2 O 0.01 g / l.

[0015] Seed liquid is cultivated in 30 ℃, 180rpm shaking table after 18 hours, inserts in the 500ml shaking flask (filling liquid volume 100ml) by 4% inoculum size, after cultivating 72 hours under the same condition, filter and collect thalli.

[0016] Use the method of grinding to crush the cells, centrifuge the cell crushing liquid with a high-speed refrigerated centrifuge (12,000rpm, 30min), collect the supernatant, slowly add an equal volume of refrigerated acetone under ice bath conditions, continue to stir for 30 minutes, and then use a high-speed refrigerated centrifuge After centrifugation, the precipitate is vacuum freeze-dried to obtain the Fusarium crude enzyme preparation.

Embodiment 2

[0018] In the 100ml grinding mouth Erlenmeyer flask, add successively the crude enzyme that 600mg makes in the embodiment 1, 60mg ginsenoside Rb 1 , then add 30ml of acetate buffer (NaAc / HAc, 0.2M, pH 5.0), plug the ground plug tightly, seal it with raw material tape, react on a rotary shaker at 200rpm at 50°C for 72 hours, and take a sample for HPLC Analysis (detection: UV 203nm; mobile phase: methanol / water=85 / 15, v / v), the conversion rate was about 30.5%.

Embodiment 3

[0020] In the 100ml grinding mouth Erlenmeyer flask, add successively the crude enzyme that 300mg makes in the embodiment 1, 60mg ginsenoside Rb 1 , then add 30ml of acetate buffer solution (NaAc / HAc, 0.2M, pH 5.0), plug the ground plug tightly, seal it with raw material tape, react on a rotary shaker at 200rpm at 50°C for 72 hours, and then add 300mg Crude enzyme, continue to react for 48 hours, add 30ml of n-butanol to extract 4 times respectively, collect n-butanol phase, concentrate by rotary evaporation, and separate through preparative chromatographic column (Venusil XBP C18) to obtain 16mg of ginsenoside F 2 , the conversion rate is about 43.2%, and the yield is 87%, the prepared ginsenoside F 2 The purity is ≥95%.

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Abstract

The present invention discloses a method of using enzymatic hydrolyzed ginsenoside Rb1 to prepare ginsenoside F2, which is characterized in that part of glycosyl in ginsenoside Rb1 molecule is selectively cut by microbial enzyme to generate the target product ginsenoside F2. The enzyme used by the invention is from fusariumspp. CGMCC No.1495 which can be prepared through fermentation and is a catalyst that is cheap and can be obtained easily. The method for preparing the ginsenoside F2 has the advantages of moderate reaction conditions, strong specificity, low cost, high recovery, etc. And the purity of all ginsenoside F2 is above 95 percent. The ginsenoside F2 can be applied to relative pharmaceutical industry.

Description

technical field [0001] The invention relates to a method for preparing ginsenoside F by enzymatic hydrolysis 2 The method, specifically, relates to a specific hydrolysis of ginsenoside Rb with microbial enzymes 1 Part of the sugar group in the molecule, making it into ginsenoside F 2 Methods. technical background [0002] As a world-renowned traditional Chinese medicine, ginseng has a long history of application. Ginsenosides are the main active ingredients of ginseng. So far, at least 40 kinds of saponin monomers have been isolated from ginseng. According to the different structures of saponins, ginsenosides can be divided into three types: diol type, triol type and oleanolic acid type. The aglycone structure of each type of saponin is the same, only the connected sugar side chains are different, but There are significant differences in pharmacological activity. Modern studies have shown that the sugar chains on saponins have an important impact on their biological act...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C12P33/20C12R1/77
Inventor 许建和苏金环
Owner EAST CHINA UNIV OF SCI & TECH