Controllable preparation method of Sb monocrystal nanowires in different growth directions
A growth direction, single crystal nanotechnology, applied in the direction of single crystal growth, crystal growth, single crystal growth, etc., can solve the problems of single crystal Sb nanowire arrays that have not been reported, and achieve industrial production, simple equipment, easy-to-handle effects
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Embodiment 1
[0032] 1. Preparation of porous alumina template: the porous alumina template was prepared in an oxalic acid solution with a molar concentration of 0.3M by the secondary anodic oxidation method, and the oxidation voltage was 40V to obtain an alumina template with a pore diameter of 60nm and a thickness of 45μm; Deposit a layer of 200nm thick Au film on the reverse side of the alumina template by evaporation method as the cathode;
[0033] 2. Prepare the electrolyte: first prepare the electrolyte containing C 6 h 8 o 7 and C 6 h 5 Na 3 o 7 buffered aqueous solution, buffered aqueous solution C 6 h 8 o 7 、C 6 h 5 Na 3 o 7 The concentrations are 2.88g / 150ml and 3.87g / 150ml respectively; SbCl is added to the buffered aqueous solution at a concentration of 0.68g / 150ml 3 , stirred for 1 hour using a magnetic stirrer, and 2 SO 4 Adjust the pH value of the solution to 2.0;
[0034] 3. Deposition device: A computer-controlled dual-electrode deposition device is used. Th...
Embodiment 2
[0045] Steps 1, 3, and 4 are the same as in Example 1;
[0046] Step 2, preparation of electrolyte: first prepare the electrolyte containing C 6 h 8 o 7 and C 6 h 5 Na 3 o 7 buffered aqueous solution, buffered aqueous solution C 6 h 8 o 7 、C 6 h 5 Na 3 o 7 The concentrations are 2.88g / 150ml and 3.87g / 150ml respectively; SbCl is added to the buffered aqueous solution at a concentration of 0.68g / 150ml 3 , using a magnetic stirrer to stir for 1 hour; finally adding sodium lauryl sulfate at a concentration of 0.01g / 150ml, using a magnetic stirrer to stir for 1 hour, and 2 SO 4 Adjust the pH value of the solution to 1.8;
[0047] Step 5. Electrodeposition process: Sb single crystal nanowires are prepared by using a computer-controlled double-electrode deposition device, with a pulse voltage of -3.0V and a pulse time of T on and relaxation time T off Both are 500μs. Using the pretreated porous alumina template as the cathode material and graphite as the anode, afte...
Embodiment 3
[0051] Steps 1, 3, 4, 5, and 6 are the same as in Example 2.
[0052] Step 2, preparation of electrolyte: first prepare the electrolyte containing C 6 h 8 o 7 and C 6 h 5 Na 3 o 7 buffered aqueous solution, buffered aqueous solution C 6 h 8 o 7 、C 6 h 5 Na 3 o 7 The concentrations are 2.88g / 150ml and 3.87g / 150ml respectively; SbCl is added to the buffered aqueous solution at a concentration of 0.68g / 150ml 3 , using a magnetic stirrer to stir for 1 hour; finally adding sodium dodecyl sulfate at a concentration of 0.3g / 150ml, using a magnetic stirrer to stir for 1.3 hours, and 2 SO 4 Adjust the pH of the solution to 1.9.
[0053] Figure 4 It is the XRD diffraction pattern of the Sb nanowire obtained in step 6 of embodiment 3. From Figure 4 (012), (110), (024) diffraction peaks can be seen, and the peak intensity of (012) is much greater than other peaks. This indicates that the Sb nanowires electrodeposited and grown in the porous alumina template by the met...
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