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Method for preparing Ti-Fe alloy by direct reduction of ilmenite

A technology of ilmenite and ti-fe, which is applied in photographic crafts, instruments, photographic auxiliary crafts, etc., can solve the problems of few raw material sources in the remelting method, can not meet the needs of users, and high oxygen content of ilmenite alloys, so as to improve the electrochemical performance. The effect of deoxidation efficiency, low production cost and high product quality

Inactive Publication Date: 2015-05-20
KUNMING UNIV OF SCI & TECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0006] The invention provides a method for preparing Ti-Fe alloy based on carbothermal in-situ pre-reduction-ionic liquid electrolytic reduction, the purpose of which is to solve the problem that the oxygen content of ferro-titanium alloy prepared by metallothermal reduction is too high, which cannot meet the needs of users and the raw material of remelting method Few sources, high energy consumption and high cost

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0022] (1) Using ilmenite as raw material and carbon powder as reducing agent, bond ilmenite powder, carbon powder accounting for 12% by mass of ilmenite powder and PVA accounting for 2% by mass of ilmenite powder The agent is mixed evenly, and then pressed into a block, and then calcined at 1000°C for 4 hours in a reducing atmosphere to make a block pre-reduced ilmenite electrode;

[0023] (2) With basic [Bmim]Cl -AlCl 3 The ionic liquid is used as the electrolyte, the pre-reduced ilmenite electrode obtained in step (1) is used as the cathode, graphite or other inert materials are used as the anode, and the electrolysis voltage is 3.0V and the electrolysis temperature is 80°C for 14 hours, and then the cathode is taken out , After washing and drying, the Ti-Fe alloy is obtained. The oxygen content of the Ti-Fe alloy is less than 600ppm.

Embodiment 2

[0025] (1) Using ilmenite as raw material and carbon powder as reducing agent, mix evenly ilmenite powder, water and carbon powder accounting for 7% of the mass percentage of ilmenite powder, wherein water accounts for 10% of the total mass of the mixture , and then make pellets with a diameter of 2mm, and then calcined at 1000°C for 2h in a reducing atmosphere of carbon monoxide, and finally put the pellets into a conductive titanium mesh with 120 meshes to make a pre-reduced ilmenite electrode ;

[0026] (2) Take [Bmim]PF 6 The ionic liquid is used as the electrolyte, the pre-reduced ilmenite electrode obtained in step (1) is used as the cathode, graphite or other inert materials are used as the anode, and the electrolysis voltage is 3V and the electrolysis temperature is 100°C for 14 hours, and then the cathode is taken out. After washing and drying, the Ti-Fe alloy is obtained. The oxygen content of the Ti-Fe alloy is less than 500 ppm.

Embodiment 3

[0028] (1) Using ilmenite as raw material and carbon powder as reducing agent, mix ilmenite powder, water and carbon powder accounting for 10% of the mass percentage of ilmenite powder evenly, wherein water accounts for 6% of the total mass of the mixture , and then made into pellets with a diameter of 1 mm, and then calcined at 1100 ° C for 1 h in a reducing atmosphere, and finally packed the pellets into a conductive titanium mesh with 200 meshes to make a pre-reduced ilmenite electrode;

[0029] (2) with [Bmim]NTf 2 The ionic liquid is used as the electrolyte, the pre-reduced ilmenite electrode obtained in step (1) is used as the cathode, graphite or other inert materials are used as the anode, the electrolysis voltage is 2.8V, and the electrolysis temperature is 25°C for 16 hours, and then the cathode is taken out , After washing and drying, the Ti-Fe alloy is obtained. The oxygen content of the Ti-Fe alloy is less than 500 ppm.

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Abstract

The invention provides a method for preparing Ti-Fe alloy by direct reduction of ilmenite, which comprises the steps of: based on ilmenite as a raw material and carbon powder as a reducing agent, calcining at 1000-1200 DEG C for 0.5-4h to prepare a pre-reduced ilmenite electrode, carrying out electrolysis at the electrolysis voltage of 2.8-3.2V and electrolysis temperature of 25-120 DEG C with an ionic liquid as the electrolyte, the obtained pre-reduced ilmenite electrode as the cathode and graphite or other inert materials as the anode for 12-48h, then taking out the cathode, washing and drying to obtain the Ti-Fe alloy. The obtained Ti-Fe alloy has lower oxygen content; and compared with the traditional Ti-Fe alloy preparation method, the method has the advantages that the process flow is shortened, the energy consumption is greatly reduced and clean production is realized.

Description

technical field [0001] The invention belongs to the field of nonferrous metal metallurgy, in particular to a method for directly preparing Ti-Fe alloy from ilmenite by combining carbothermal pre-reduction and ionic liquid electrolytic reduction. Background technique [0002] Ferro-titanium alloy is not only an important raw material in iron and steel smelting, but also an important magnetic material and one of the most potential hydrogen storage materials, which has a wide range of industrial applications. For example, the use of titanium-iron alloys in steelmaking can not only improve the mechanical properties of steel, but also improve its crystal structure. [0003] At present, the production of ferro-titanium alloy mainly adopts metal thermal reduction method (aluminothermic reduction method) and remelting method. Among them, the aluminothermic reduction method is to mix ilmenite concentrate powder, aluminum powder, and ferrosilicon in a certain proportion, and then use...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C25C1/24
Inventor 华一新徐存英张笑盈张启波李艳李坚
Owner KUNMING UNIV OF SCI & TECH