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Copper/manganese composited nitric oxide normal-temperature catalyst and preparation method thereof

A nitric oxide, catalyst technology, applied in catalyst activation/preparation, physical/chemical process catalyst, metal/metal oxide/metal hydroxide catalyst, etc., can solve the complex process, high reaction temperature, not suitable for NOx purification Treatment and other problems, to achieve the effect of simple process, high catalytic oxidation efficiency, and improved absorption efficiency

Inactive Publication Date: 2014-02-12
SHANGHAI NAT ENG RES CENT FORNANOTECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0004] In the research on the catalytic oxidation of nitric oxide, some literatures disclose a kind of mesoporous silica as the carrier, one or two mixtures of potassium and molybdenum as the doping component, and platinum as the active component. Catalyst for catalytic oxidation of nitrogen oxides in flue gas prepared by impregnation method, but the process is more complicated, and the reaction temperature is higher at 150-300 °C
There is a document disclosing a flue gas catalytic oxidation denitrification process, using TiO 2 or ZrO 2 -TiO 2 As the carrier, Co is the catalyst of the active component, but also the reaction temperature is too high, so it is not suitable for NOx purification treatment under normal temperature conditions

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0017] Weigh 0.02mol manganese acetate and copper chloride respectively, dissolve them in 5ml deionized water, add appropriate amount of citric acid until the solution pH=4;

[0018] Weigh 0.04mol ammonium chloride at the ratio of metal ion: ammonium chloride = 1:1 (molar ratio), mix it with the metal salt solution evenly, and let it stand for 6-8 hours;

[0019] Weigh 3.25 g of 20-40 mesh activated alumina powder; immerse the alumina powder in the above solution at room temperature and equal volume for 12 hours, and then dry it in an oven at 120°C for 8 hours;

[0020] The nitric oxide catalyst can be obtained by calcining the above alumina powder in a muffle furnace at 450° C. for 3 hours.

[0021] The catalytic performance of the prepared catalyst was evaluated according to the aforementioned test conditions, and the catalytic conversion rate of NO was determined to be 95%, and the catalytic effect was basically stable within 3 hours.

Embodiment 2

[0023] Weigh 0.02mol of manganese acetate and 0.01mol of copper chloride respectively, dissolve them in 5ml of deionized water, add an appropriate amount of citric acid until the solution pH=4;

[0024] Weigh 0.03mol ammonium chloride at the ratio of metal ion: ammonium chloride = 1:1 (molar ratio), mix it with the metal salt solution evenly, and let it stand for 6-8 hours;

[0025] Weigh 3.25, 20-40 mesh activated alumina powder; immerse the alumina powder in the above solution at room temperature and equal volume for 12 hours, and then dry it in an oven at 120°C for 8 hours;

[0026] The nitric oxide catalyst can be obtained by calcining the above alumina powder in a muffle furnace at 450° C. for 3 hours.

[0027] The catalytic performance of the prepared catalyst was evaluated according to the aforementioned test conditions. It was determined that the catalytic conversion rate of NO was 90%, and the catalytic effect was basically stable within 3 hours.

Embodiment 3

[0029] Weigh 0.005mol manganese acetate and 0.02mol copper chloride respectively, dissolve them in 5ml deionized water, add appropriate amount of citric acid until the solution pH=4;

[0030] Weigh 0.0375mol ammonium chloride at the ratio of metal ion:ammonium chloride=1:1.5 (molar ratio), mix it with the metal salt solution evenly, and let it stand for 6-8 hours;

[0031] Weigh 3.25 g of 20-40 mesh activated alumina powder; impregnate the alumina powder in the above solution at room temperature for 12 hours, and then dry it in an oven at 120°C for 8 hours;

[0032] The nitric oxide catalyst can be obtained by calcining the above-mentioned alumina powder in a muffle furnace at 400° C. for 5 hours.

[0033] The catalytic performance of the prepared catalyst was evaluated according to the aforementioned test conditions, and the catalytic conversion rate of NO was determined to be 86%, and the catalytic effect was basically stable within 3 hours.

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Abstract

The invention discloses a copper / manganese composited nitric oxide normal-temperature catalyst. The catalyst is characterized in that the catalyst comprises 50-85% by weight of aluminum oxide and 15-50% by weight of a metal oxide. The invention discloses a preparation method of the copper / manganese composited nitric oxide normal-temperature catalyst. The method is characterized in that: active aluminum oxide power is used as a carrier, citric acid and an ammonium salt are used as auxiliary agents, manganese acetate and cupric chloride are dipped and loaded respectively through an isopyknic method, and a metal oxide with high activity is synthesized on the surface of the aluminum oxide after sintering, thus obtaining the copper / manganese composited nitric oxide normal-temperature catalyst. The method has characteristics of simple preparation technology, high efficiency for catalytic oxidation, and the like.

Description

technical field [0001] The invention relates to a catalyst for catalytic oxidation of nitrogen monoxide under normal temperature and normal pressure environment and its preparation method, in particular to a copper-manganese composite nitrogen monoxide catalyst at normal temperature and its preparation method, which is applied to the field of environmental purification for the treatment of NOx gas pollutants . Background technique [0002] Among various air pollutants, NO X pollution and the harm it causes cannot be ignored. Most of NOx comes from fuel combustion, that is, vehicle exhaust, industrial kiln emissions, etc. NOx purification treatment can be divided into dry method and wet method according to the process. Dry methods include non-catalytic reduction methods, catalytic reduction methods, adsorption methods, etc.; wet methods include acid absorption, alkali absorption, oxidation absorption, etc. [0003] Oxidation and absorption of NOx under oxygen-enriched con...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): B01J23/889B01J37/02B01D53/86B01D53/56
Inventor 张豪杰董亚梅何丹农
Owner SHANGHAI NAT ENG RES CENT FORNANOTECH