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Preparation method of hydrocracking catalyst

A hydrocracking and catalyst technology, applied in physical/chemical process catalysts, molecular sieve catalysts, chemical instruments and methods, etc., can solve problems such as high reaction temperature, low activity, poor raw material adaptability, etc.

Active Publication Date: 2014-05-14
CHINA PETROLEUM & CHEM CORP +1
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Although this catalyst can also be used as a medium-oil type hydrocracking catalyst, due to the characteristics of the β zeolite used, the content range of β zeolite in the medium-oil type catalyst is generally limited to 2.5w%-10w%, and generally must be used together A dispersed in γ-Al 2 o 3 Such as silica-alumina on a macroporous alumina substrate, the medium-oil catalyst involved in this patent has to lower the activity in order to ensure the selectivity of medium-oil, so that the reaction temperature is relatively high, generally above 390 ° C, which leads to poor raw material adaptability

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0032] The carrier T-1 of Comparative Example 1 was impregnated with an impregnation solution containing tungsten and nickel at room temperature for 2 hours, and dried at 120°C for 4 hours to prepare dimethylhydrazine NH with a concentration of 30% by weight. 2 N(CH 3 ) 2 Solution, the above-mentioned dried material is impregnated with the prepared solution for 2 hours, dried at 100°C for 4 hours, heat-treated at 250°C for 6 hours in an air atmosphere, and then reduced and activated under a hydrogen atmosphere. The reduction and activation procedure is as follows: Raise from room temperature to 450°C at 5°C / min, from 450°C to 500°C at a heating rate of 2°C / min, and keep at 500°C for 2 hours to prepare catalyst C-1 of the present invention.

Embodiment 2

[0037] The carrier T-2 of Comparative Example 2 was impregnated with an impregnation solution containing tungsten compound and nickel compound for 2 hours at room temperature, and dried at 100°C for 6 hours to prepare dimethylhydrazine NH with a weight concentration of 40%. 2 N(CH 3 ) 2 solution, the above-mentioned dried carrier was impregnated with the prepared solution for 2 hours, dried at 100°C for 5 hours, heat-treated at 400°C for 1 hour in an air atmosphere, and then activated with hydrogen in a hydrogen atmosphere. °C / min was raised from room temperature to 350 °C, at a rate of 1 °C / min, from 350 °C to 500 °C, and kept at 500 °C for 4 hours to prepare transition metal phosphide catalyst C-2.

Embodiment 3

[0042] The carrier T-3 of Comparative Example 3 was impregnated with an impregnation solution containing tungsten and nickel at room temperature for 2 hours, and dried at 110°C for 6 hours to prepare dimethylhydrazine NH with a weight concentration of 60%. 2 N(CH 3 ) 2 solution, the above-mentioned dried carrier was impregnated with the prepared solution for 2 hours, dried at 110°C for 5 hours, heat-treated at 350°C for 2 hours in an air atmosphere, and then activated under a hydrogen atmosphere. °C / min was raised from room temperature to 450 °C, at a rate of 1 °C / min, from 450 °C to 500 °C, and kept at 500 °C for 4 hours to prepare transition metal phosphide catalyst C-3.

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PUM

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Abstract

The present invention discloses a preparation method of a hydrocracking catalyst. The method includes the following steps: (1) preparing a catalyst carrier containing a molecular sieve and an inorganic refractory oxide; (2) preparing a dipping solution containing a group VI metallic compound B and / or group VIII metallic compound; (3) dipping the catalyst carrier obtained in the step (1) with the dipping solution prepared in the step (2), and then drying the carrier; (4) preparing a hydrazine derivative solution and dipping the materials obtained in the step (3) in the hydrazine derivative solution, and then drying; (5) performing a heat treatment at 200-450 DEG C in the air atmosphere to the materials obtained in the step (4) for 1-6 h; and (6) activating the materials obtained in the step (5) after the heat treatment by using hydrogen, so as to obtain the hydrocracking catalyst used for the hydrocracking reaction after the activation. The hydrocracking catalyst provided by the invention can be used for the treatment of heavy hydrocarbon materials and can produce middle distillates by the maximum.

Description

technical field [0001] The invention relates to a method for preparing a hydrocracking catalyst. The catalyst has excellent hydrocracking performance, high activity and high selectivity for medium oil. Background technique [0002] The hydrocracking catalyst is a dual-functional catalyst with hydrogenation and cracking properties. Non-precious metal hydrocracking catalysts generally use Group VIB and Group VIII metals as hydrogenation components, and the cracking performance is mainly provided by acidic components. Crystalline zeolite and / or amorphous silica-alumina can be used. Simple use of amorphous silica-alumina, although the selectivity is high, but the activity is low, and the flexibility of operation is limited. In most hydrocracking catalysts, crystalline zeolite is used as the acidic component, or crystalline zeolite and amorphous Silica and aluminum are common acidic components. [0003] Most of the medium-oil hydrocracking catalysts currently used in industrial...

Claims

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Application Information

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IPC IPC(8): B01J29/16B01J29/78C10G47/20C10G65/12
Inventor 谷明镝王刚曹春清卜岩白振民黄薇
Owner CHINA PETROLEUM & CHEM CORP