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Preparation method and application of a ractopamine electrochemical bioimmunosensor

A technology of ractopamine and biological immunity, which is applied in the direction of chemiluminescence/bioluminescence, electrochemical variables of materials, and analysis by making materials undergo chemical reactions, can solve the problems affecting the convenience of operation and restricting wide application, etc., to achieve Easy operation, high selectivity detection, simple preparation effect

Inactive Publication Date: 2017-05-31
UNIV OF JINAN
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0007] However, since the electrochemiluminescence sensor requires external light signal capture devices such as photodiodes, and the photoelectrochemical sensor requires an external light source to excite the photosensitive material, this affects the convenience of the operation of the two to a certain extent and limits them. Wider application in actual production and life

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0041] Example 1 A ractopamine electrochemical bioimmunosensor, the specific preparation steps are:

[0042] (1) Preparation of ECL working electrode W1:

[0043] 1) Use ITO conductive glass as the working electrode, and drop-coat NH on the surface of the electrode 4 NiPO 4 Solution, covering an area of ​​1 cm × 1 cm, dry at room temperature;

[0044] 2) Apply the working electrode obtained in 1) to the NH 4 NiPO 4 Surface drop coating of Au@Ag 2 S NRs sol, covering an area of ​​1 cm × 1 cm, dried at room temperature;

[0045] 3) Immerse the working electrode obtained in 2) into the electrolyte, and the immersion area is NH 4 NiPO 4 and Au@Ag 2 The area covered by S NRs was electrochemically deposited on the working electrode using a three-electrode system. After deposition, the working electrode was taken out, washed with ultrapure water, and dried at 4 °C in the dark to prepare the electrochemiluminescence working electrode W1;

[0046] The NH 4 NiPO 4 The solutio...

Embodiment 2

[0064] Example 2 A ractopamine electrochemical bioimmunosensor, the specific preparation steps are:

[0065] (1) Preparation of ECL working electrode W1:

[0066] The preparation steps are the same as the preparation steps of W1 in Example 1, the difference is: the ammonium salt addition is 0.3 g in the preparation step of the nickel ammonium phosphate micro-nano material, the phosphate addition is 0.20 g, and the nickel dichloride addition is 0.20 g, the stirring temperature and time were 38 ℃ and 12 h, respectively; the length of gold nanorods was 30 nm; the concentration of luminol in the electrolyte was 5 mmol / L, and the concentration of sulfuric acid was 0.5 mol / L; cyclic voltammetry When performing electrochemical deposition, cycle 25 times;

[0067] (2) Preparation of photoelectrochemical working electrode W2:

[0068] 1) Use ITO conductive glass as the working electrode, drop-coat 10 µL TiO on the surface of the electrode 2 NSs sol, dry at room temperature;

[006...

Embodiment 3

[0074] Example 3 A ractopamine electrochemical bioimmunosensor, the specific preparation steps are:

[0075] (1) Preparation of electrochemiluminescence working electrode W1:

[0076] The preparation steps are the same as the preparation steps of W1 in Example 1, the difference is: the ammonium salt addition is 0.4 g in the preparation step of the nickel ammonium phosphate micro-nano material, the phosphate addition is 0.25 g, and the nickel dichloride addition is 0.25 g, the stirring temperature and time were 45 ℃ and 14 h, respectively; the length of gold nanorods was 40 nm; the concentration of luminol in the electrolyte was 10 mmol / L, and the concentration of sulfuric acid was 1.0 mol / L; cyclic voltammetry When performing electrochemical deposition, cycle 30 times;

[0077] (2) Preparation of photoelectrochemical working electrode W2:

[0078] 1) Using ITO conductive glass as the working electrode, drop-coat 12 µL TiO on the surface of the electrode 2 NSs sol, dry at r...

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Abstract

The invention discloses a preparation method of a bioimmune sensor with dual signal development strategies of electrochemiluminescence and photoelectrochemistry constructed on the basis of functional nanomaterials. The prepared sensor is simple to operate, easy to carry, fast to detect, and low in cost, and can be used in Rapid and sensitive detection of ractopamine in daily production and daily life.

Description

technical field [0001] The invention relates to a preparation method of a telephonic bioimmune sensor for detecting ractopamine. The sensor integrates dual functions of electrochemiluminescence and photoelectrochemistry. It belongs to the field of new nano functional materials and electrochemical biosensing analysis technology. Background technique [0002] Ractopamine is a synthetic β-adrenoceptor agonist of clonopamine, which is used by some pig farms as a new type of clenbuterol. Because eating a large amount of meat or offal containing ractopamine residues may cause people to have symptoms of poisoning such as dyspnea, nausea, dizziness, heart palpitations, and increased blood pressure. In severe cases, it will affect the reproductive system. Therefore, the use of ractopamine has been banned in China since February 5, 2013. [0003] At present, the methods for detecting ractopamine mainly include chromatography and mass spectrometry. Such methods require expensive ins...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): G01N33/543G01N21/76G01N27/30G01N27/327
CPCG01N21/76G01N27/305G01N27/327G01N33/54306G01N33/54386
Inventor 张勇魏琴杜斌马洪敏范大伟
Owner UNIV OF JINAN