Copolyester for environmentally-friendly tin printing ink and preparation method thereof
A technology of iron printing ink and copolyester, which is applied in the field of environment-friendly copolyester for iron printing ink and its preparation, can solve problems such as non-compliance with environmental protection, and achieve the effects of convenient industrial production, high adhesion and good bonding performance
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[0026] The preparation method step of above-mentioned copolyester is as follows:
[0027] (1) Esterification reaction:
[0028] Add diols and dicarboxylic acid monomers with an alkyd molar ratio (1.1~1.8): 1.0 into the polymerization reactor, add a certain proportion of catalyst and heat stabilizer, at 200°C~250°C, 0~0.3 The esterification reaction is carried out under MPa for 2 to 4 hours, and the esterification reaction is completed when the esterification water output reaches the theoretical value. Wherein, the added amount of the catalyst is 0.01%-0.1% of the total mass of the copolyester; the added amount of the heat stabilizer is 0.01%-0.08% of the total mass of the polyester.
[0029] Wherein, the added dicarboxylic acid monomer is one or more of terephthalic acid, isophthalic acid, adipic acid, sebacic acid and succinic acid; One or more of alcohol, neopentyl glycol, 1,4-cyclohexanedimethanol, 2-methyl-1,3-propanediol; the catalyst is antimony trioxide, antimony acet...
Embodiment 1
[0034] Example 1: In a 20-liter polymerization reactor, add purified terephthalic acid, isophthalic acid, adipic acid, ethylene glycol, neopentyl glycol, 1,4-cyclo Hexanedimethanol. Among them, the ratio of purified terephthalic acid to the total moles of dicarboxylic acids is 65%, the ratio of isophthalic acid to the total moles of dicarboxylic acids is 25%, and the ratio of adipic acid to the total moles of dicarboxylic acids is 65%. The proportion of ethylene glycol is 10%; the proportion of ethylene glycol to the total moles of diols is 74%, the proportion of neopentyl glycol to the total moles of diols is 20%, and the proportion of 1,4-cyclohexanedimethanol to The total molar ratio of dihydric alcohol is 6%, and 2 g of ethylene glycol antimony is added. Nitrogen replacement, temperature rise, esterification reaction at 200°C-250°C, 0.0-0.3MPa, when the esterification water output reaches the theoretical value, the esterification stage ends. Release to normal pressure, a...
Embodiment 2
[0035] Embodiment two: adopt the same raw material ratio and catalyst addition as in embodiment one, only adjust the addition of SIPE to be 8% of the copolyester quality, carry out polymerization test under the technological conditions of embodiment one, obtain certain intrinsic viscosity copolyester.
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