Organic light-emitting device and display device
An electroluminescent device and electroluminescent technology are applied in the fields of organic electroluminescent devices, display devices, and biindole materials, which can solve the problems of low utilization rate, high technical content and high energy consumption, and achieve the reduction of driving voltage, Improved luminous efficiency and good film-forming properties
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Embodiment 1
[0036] The synthesis of embodiment 1 compound P-1:
[0037]
[0038] In a 500ml three-necked flask, under nitrogen protection, add 300ml of dry toluene, 19.2g (0.05mol) of 3,3'-diphenyl-1H,1'H-2,2'-biindole, 38.9g (0.12mol) 4-bromotriphenylamine, 14.4 grams (0.15mol) of sodium tert-butoxide, 0.58 grams (0.001mol) of bis(dibenzylideneacetone) palladium, 2.02 grams (0.001mol) of 10% tri-tert-butyl The toluene solution of phosphine was heated to reflux for 8 hours and then lowered to room temperature, dilute hydrochloric acid was added, the layers were separated, the organic layer was washed with water until neutral, dried with anhydrous magnesium sulfate, separated by silica gel column, ethyl acetate: petroleum ether =1:5 (volume ratio) elution, the eluate was concentrated to dryness, and recrystallized from methanol / toluene mixed solvent to obtain 33.8 g of the compound represented by formula P-1 with a yield of 77.61%.
[0039] Mass spectrometry was performed on the obtain...
Embodiment 2
[0042] Synthesis of other part compounds of embodiment 2
[0043] Referring to the synthesis method of compound P-1, only the 4-bromotriphenylamine in it is replaced by the corresponding bromoarylamine as required, and other compounds shown in the compound of the present invention can be synthesized.
[0044] The following table lists the brominated aromatic amines used in the specific reactions of some compounds and the resulting product mass spectrometry data list as follows:
[0045]
[0046]
[0047]
[0048]
[0049] According to another aspect of the present invention, an organic electroluminescent device is provided, the hole injection material / hole transport material of the organic electroluminescent device is the biindoles containing triarylamine groups according to the present invention Material.
[0050] The typical structure of an organic electroluminescent device is: substrate / anode / hole injection layer / hole transport layer (HTL) / organic light-emitting ...
Embodiment 3
[0063] The compound of the present invention is used as the hole transport material in the organic electroluminescent device, and as a comparative organic electroluminescent device, the hole transport material is NPB.
[0064] The structure of the organic electroluminescence device is: ITO / HIL02 (100nm) / HTL (40nm) / EM1 (30nm) / ETL (20nm) / LiF (0.5nm) / Al (150nm).
[0065] In the production of the organic electroluminescent device in this embodiment, a glass substrate is selected, ITO is used as the anode material, HIL02 is used as the hole injection layer, EM1 is used as the main material of the organic light-emitting layer, TAZ is used as the electron transport layer material, and LiF / Al is used as the electron injection layer. layer / cathode material.
[0066] The preparation process of the organic electroluminescent device in this embodiment is as follows:
[0067] The glass substrate coated with the ITO transparent conductive layer (as the anode) is ultrasonically treated in a...
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