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Mixed material for preparing polyethersulfone hollow fiber membrane and preparation method and application

A technology of mixed materials and polyethersulfone, applied in chemical instruments and methods, membrane technology, semi-permeable membrane separation, etc., can solve the problems of poor hydrophilic stability and easy washing out, and achieve good biocompatibility and Effects of anti-fouling, hard to wash off, stable hydrophilicity and water wettability

Active Publication Date: 2022-01-04
SHENZHEN ZHONGXING NEW MATERIAL TECH CO LTD
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

This excellent performance makes it popular among membrane material modification workers, but polyvinylpyrrolidone is easily soluble in water, and it is easy to wash out, resulting in poor hydrophilic stability of the membrane.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0047] The mixed material of this example is mixed by the weight ratio of modified polyvinylpyrrolidone:polyethersulfone=1:15, wherein the modified polyvinylpyrrolidone is formed by the micro-crosslinking reaction of chitosan and polyvinylpyrrolidone. The mixed materials were prepared to obtain the polyethersulfone hollow fiber membrane of this example. Concrete, the preparation method of modified polyvinylpyrrolidone and polyethersulfone hollow fiber membrane is as follows:

[0048] Preparation of modified polyvinylpyrrolidone: dissolve 100g chitosan in 2.5L acetic acid solution, add 1400g polyvinylpyrrolidone, add 12g cerium amine nitrate while stirring at 60°C, add 10g glyoxal and cerium nitrate after cooling to room temperature The mass ratio of amine to glyoxal is 1.2:1. Stir evenly and heat up to 60°C, react for 4 hours, wash the reaction product with 2wt% acetic acid, isopropanol, and ultrapure water, and dry at 100°C to obtain modified polyvinylpyrrolidone, that is, c...

Embodiment 2

[0053] The mixed material of this example is mixed by the weight ratio of modified polyvinylpyrrolidone: polyethersulfone = 1:9, wherein the modified polyvinylpyrrolidone is formed by the micro-crosslinking reaction of chitosan and polyvinylpyrrolidone. The mixed materials were prepared to obtain the polyethersulfone hollow fiber membrane of this example. Concrete, the preparation method of modified polyvinylpyrrolidone and polyethersulfone hollow fiber membrane is as follows:

[0054] Preparation of modified polyvinylpyrrolidone: 100g chitosan was dissolved in 2.5L acetic acid solution, 500g polyvinylpyrrolidone was added, 27g cerium sulfate was added while stirring at 60°C, and 18g glutaraldehyde was added after cooling to room temperature. Stir evenly and heat up to 60°C, react for 5 hours, wash the reaction product with 2wt% acetic acid, isopropanol, and ultrapure water, and dry at 100°C to obtain modified polyvinylpyrrolidone.

[0055] Preparation of polyethersulfone hol...

Embodiment 3

[0058] The mixed material of this example is mixed by the weight ratio of modified polyvinylpyrrolidone:polyethersulfone=1:18, wherein the modified polyvinylpyrrolidone is formed by the micro-crosslinking reaction of chitosan and polyvinylpyrrolidone. The mixed materials were prepared to obtain the polyethersulfone hollow fiber membrane of this example. Concrete, the preparation method of modified polyvinylpyrrolidone and polyethersulfone hollow fiber membrane is as follows:

[0059] Preparation of modified polyvinylpyrrolidone: Dissolve 100g chitosan in 2.5L formic acid solution, add 2000g polyvinylpyrrolidone, add 32.5g cerium amine sulfate while stirring at 60°C, add 25g subaldehyde and cerium nitrate after cooling to room temperature The mass ratio of amine to glyoxal is 1.3:1. Stir evenly and heat up to 60°C, react for 4 hours, wash the reaction product with 2wt% acetic acid, isopropanol, and ultrapure water, and dry at 100°C to obtain modified polyvinylpyrrolidone.

[...

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Abstract

The application discloses a mixed material for preparing a polyethersulfone hollow fiber membrane, a preparation method and an application. The mixed material used in the preparation of polyethersulfone hollow fiber membranes in the present application includes uniformly mixed polyethersulfone and modified polyvinylpyrrolidone, wherein the modified polyvinylpyrrolidone is a micro-crosslinked product of polyvinylpyrrolidone and chitosan. The mixed material and the polyethersulfone hollow fiber membrane of the present application are micro-crosslinked by polyvinylpyrrolidone and chitosan, so that the polyvinylpyrrolidone is not easy to elute, and the film-forming property is good after blending with polyethersulfone. The modified polyethersulfone hollow fiber membrane has stable chemical properties, heat resistance, stable hydrophilicity and water wettability, and good biocompatibility and fouling resistance.

Description

technical field [0001] The application relates to the field of polyethersulfone hollow fibers, in particular to a mixed material for preparing polyethersulfone hollow fiber membranes and its preparation method and application. Background technique [0002] Polyethersulfone is a thermoplastic polymer material with excellent performance, which has excellent physical and chemical properties such as heat resistance, acid resistance, alkali resistance, oxidation resistance, etc. At present, hollow fiber membranes prepared from polyethersulfone, that is, polyethersulfone hollow fiber membranes, are widely used in the fields of water treatment and blood purification. Since polyethersulfone is a hydrophobic material, it needs to be modified by hydrophilicity when it is used in the field of medical blood purification to enhance its water wettability. [0003] At present, the conventional hydrophilic modification method for polyethersulfone hollow fiber membranes is to introduce poly...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B01D71/76B01D71/68B01D69/08B01D67/00A61M1/16C02F1/44
CPCB01D71/68B01D71/76B01D69/08B01D67/0002A61M1/16C02F1/44
Inventor 肖智贤曹志锋丁云海
Owner SHENZHEN ZHONGXING NEW MATERIAL TECH CO LTD