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A kind of preparation method of cattail velvet fiber lithium-ion battery diaphragm

A cattail velvet fiber and lithium-ion battery technology, applied in the field of electrochemistry, can solve the problems of low porosity of the diaphragm, complicated preparation process, and low mechanical strength, and achieve the effects of improved mechanical properties, simple process flow, and low equipment requirements

Active Publication Date: 2021-11-16
WUHAN TEXTILE UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

However, the biomass cellulose porous composite diaphragm obtained by the appeal method has the following main disadvantages: low mechanical strength, low porosity of the diaphragm, high production cost, complicated preparation process, and low yield

Method used

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Examples

Experimental program
Comparison scheme
Effect test

preparation example Construction

[0017] A kind of preparation method of cattail velvet fiber lithium-ion battery diaphragm, described preparation method is carried out according to the following steps:

[0018] A. Cattail velvet fiber pretreatment

[0019] At room temperature, put 2g of cattail velvet fibers in a mixed solution of deionized water and ethanol with a mass ratio of 1:1, wash three times to remove impurities, and then dry at 80°C for 6h; take out the dried cattail velvet fibers and place In the solution prepared by mixing 1g of chlorine oxysalt and 100ml of deionized water, use acetic acid to adjust the pH value of the solution to 4.5, and then stir at 80°C for 1h; after the stirring, the collected cattail fibers, Wash three times in a mixed solution of deionized water and ethanol with a mass ratio of 1:1, and then dry at 80°C for 4 hours to obtain pretreated cattail velvet fibers.

[0020] B. Cattail velvet fiber oxidation treatment

[0021] Mix 0.016~0.048g of 2,2,6,6-tetramethylpiperidine-1-...

Embodiment 1

[0030] A. Cattail velvet fiber pretreatment

[0031] At room temperature, put 2g of cattail velvet fibers in a mixed solution of deionized water and ethanol with a mass ratio of 1:1, wash three times to remove impurities, and then dry at 80°C for 6 hours; take out the dried cattail velvet fibers and place them in In the solution prepared by mixing 1g of chlorine oxysalt and 100ml of deionized water, use acetic acid to adjust the pH value of the solution to 4.5, and then stir at 80°C for 1h; Wash three times in a mixed solution of deionized water and ethanol with a mass ratio of 1:1, and then dry at 80°C for 4 hours to obtain pretreated cattail velvet fibers.

[0032] B. Cattail velvet fiber oxidation treatment

[0033] Mix 0.016g of 2,2,6,6-tetramethylpiperidine-1-oxyl radical with 0.1g of NaBr into 100ml of deionized water, stir until completely dissolved, and mix with the pretreated cattail velvet in step A Mix the fibers, slowly add 8ml of 0.6mol / L NaClO solution, use NaO...

Embodiment 2

[0038] A. Cattail velvet fiber pretreatment

[0039] At room temperature, put 2g of cattail velvet fibers in a mixed solution of deionized water and ethanol with a mass ratio of 1:1, wash three times to remove impurities, and then dry at 80°C for 6 hours; take out the dried cattail velvet fibers and place them in In the solution prepared by mixing 1g of chlorine oxysalt and 100ml of deionized water, use acetic acid to adjust the pH value of the solution to 4.5, and then stir at 80°C for 1h; Wash three times in a mixed solution of deionized water and ethanol with a mass ratio of 1:1, and then dry at 80°C for 4 hours to obtain pretreated cattail velvet fibers.

[0040] B. Cattail velvet fiber oxidation treatment

[0041]Mix 0.032g of 2,2,6,6-tetramethylpiperidine-1-oxyl radical with 0.2g of NaBr into 100ml of deionized water, stir until completely dissolved, and mix with the pretreated cattail velvet in step A Mix the fibers, slowly add 8ml of 0.6mol / L NaClO solution, use NaOH...

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Abstract

The invention relates to the preparation of a lithium-ion battery diaphragm, in particular to a preparation method of a cattail velvet fiber lithium-ion battery diaphragm. It belongs to the field of electrochemical technology. The present invention pretreats the picked cattail fibers, then oxidizes them at room temperature through a 2,2,6,6-tetramethylpiperidine-1-oxyl free radical / NaBr / NaClO mixed oxidation system, and then centrifuges and cleans them. Finally, 2,2,6,6-tetramethylpiperidine-1-oxyl free radical oxidation cattail fibers are obtained, and the oxidized cattail fibers are mixed with organic solvents to obtain cattail fiber lithium-ion battery separator precursors The solution is then suction-filtered and dried to produce a battery diaphragm with a thickness less than 50 microns and a porosity greater than 80%. The cattail velvet fiber lithium-ion battery diaphragm prepared by the invention has the characteristics of high mechanical strength, good wettability, good thermal stability, high porosity and high ion conductivity, and is beneficial to the industrialized production of new power batteries. The preparation method of the present invention has the characteristics of simple technological process, low equipment requirements, low cost and suitable for industrialized production.

Description

technical field [0001] The invention relates to the preparation of a lithium-ion battery diaphragm, in particular to a preparation method of a cattail velvet fiber lithium-ion battery diaphragm, and belongs to the technical field of electrochemistry. Background technique [0002] The separator is one of the important components of lithium-ion batteries. Most of the commercial separators used today are polyolefin separators. Although they have good chemical stability and inherent shutdown function, they also have poor thermal stability and limited wettability. And other defects, and plant fibers have good chemical stability, excellent thermal stability, high dielectric constant and other excellent properties. Therefore, biomaterials such as plant fibers with high safety and low cost are used to prepare lithium-ion battery separators. [0003] Cattail velvet fiber is a natural plant fiber with rich resources and great development potential. Its mass specific resistance is muc...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): H01M50/403H01M50/44H01M10/0525
CPCH01M10/0525H01M50/403H01M50/411H01M50/44Y02E60/10
Inventor 许杰黄成豪范玲玲纪辉杨源徐卫林包海峰
Owner WUHAN TEXTILE UNIV