A kind of hydrophilic polysiloxane copolymer and its preparation method and application, wear-resistant self-lubricating anti-fog coating and its preparation method
A technology of siloxane copolymer and polysiloxane, applied in the field of materials, can solve the problems of complexity and poor mechanical wear resistance, and achieve the effects of easy scale-up production, lower friction coefficient and good application prospects.
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[0041] The present invention also provides the preparation method of the hydrophilic polysiloxane copolymer described in the above technical scheme, comprising the following steps:
[0042] α-Butyldimethylsiloxane-ω-3-methacryloxypropylene polysiloxane and hydrophilic monomers are polymerized under a free radical initiator to obtain a compound having the structure shown in formula I Hydrophilic polysiloxane copolymer; the hydrophilic monomer is 3-sulfonic acid propyl methacrylate potassium salt, dimethylaminoethyl methacrylate, dimethyl butyl ammonium bromide Or [2-(methacryloyloxy)ethyl]dimethyl-(3-sulfopropyl)ammonium hydroxide.
[0043] The present invention has no special limitation on the sources of the α-butyldimethylsiloxane-ω-3-methacryloxypropylene polysiloxane and hydrophilic monomers, and adopts methods well known to those skilled in the art. The preparation method or purchase of commercially available products, specifically, α-butyldimethylsiloxane-ω-3-methacrylox...
Embodiment 1
[0059] (1) Take α-butyldimethylsiloxane-ω-3-methacryloxypropyl polysiloxane 10g (number average molecular weight 1000), dimethylaminoethyl methacrylate 14.3g, azo Add 0.24 g of diisobutyronitrile and 20 g of xylene as a solvent into a three-necked flask. After purging with nitrogen for 20 minutes, heat up to 85° C. and react for 5 hours to obtain a hydrophilic polysiloxane copolymer solution.
[0060] (2) Precipitate the polymer with n-hexane from the copolymer solution obtained above, and dry it to obtain a pure hydrophilic polysiloxane copolymer.
[0061] (3) Dilute the above polymer with ethanol to a mass concentration of 1% for later use.
[0062] (4) After the PET substrate is ultrasonically cleaned with ethanol, it is dried at room temperature for later use.
[0063] (5) Spin-coat the polymer solution in step (2) on the above-mentioned clean PET substrate, the spin-coating process: the rotation speed is 500 rpm, and the time is 30 seconds.
[0064] (6) Remove the PET f...
Embodiment 2
[0068] (1) Get α-butyl dimethyl siloxane-ω-3-methacryloxypropyl polysiloxane 10g (number average molecular weight 1000), dimethyl butyl ammonium bromide 15.8g , 0.24g of azobisisobutyronitrile and 20g of xylene as a solvent were added to a three-necked flask. After purging with nitrogen for 20 minutes, the temperature was raised to 85°C and reacted for 5 hours to obtain a hydrophilic polysiloxane copolymer solution.
[0069] (2) Precipitate the polymer with n-hexane from the copolymer solution obtained above, and dry it to obtain a pure hydrophilic polysiloxane copolymer.
[0070] (3) Dilute the above polymer with ethanol to a mass concentration of 1% for later use.
[0071] (4) After the PET substrate is ultrasonically cleaned with ethanol, it is dried at room temperature for later use.
[0072] (5) Spin-coat the polymer solution in step (2) on the above-mentioned clean PET substrate, the spin-coating process: the rotation speed is 500 rpm, and the time is 30 seconds.
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