A compound for organic light-emitting and its application
A compound and organic technology, applied in the field of organic light-emitting compounds, can solve the problems of reduced efficiency and lifespan, the service life of TADF devices does not meet the display application industry standards, and the display application is not expected. Transport properties, effects of excellent hole and electron transport properties
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Embodiment
[0028] This embodiment provides the above-mentioned preparation method for the organic light-emitting compound.
[0029] ① Synthetic intermediates:
[0030]
[0031] Raw material (10mmol), p-dibromobenzene (8mmol, log) are added to the two-necked flask of 100mL, under nitrogen conditions, cuprous iodide (0.6mmol), potassium carbonate (10mmol), 1,10-o-phenanthroline ( 0.6 mmol), 50 mL of DMF, reacted at 155 °C for 48 hours; the mixture was extracted three times with ethyl acetate; the extract was washed with MgSO 4 dried, filtered, concentrated and subjected to column chromatography (silica gel, from 100:1 PE / CH 2 Cl 2 to 5:1PE / CH 2 Cl 2 gradient elution) to give a white solid.
[0032]
[0033] The above-mentioned white solid (10 mmol) was added to a two-necked flask of 100 mL, 30 mL of acetic acid was added, and 3 times the amount of hydrogen peroxide was added, and the temperature was raised to reflux for 2 hours; 4 dried, filtered, concentrated and subjected to ...
specific Embodiment 1
[0038]
[0039] Further purification using reverse phase column chromatography with acetonitrile as eluent gave a white solid and its structure was determined by mass spectrometry, HRMS Calcd for C 38 H 24 N 2 O 2 S: 572.16, Found: 572.14. Theoretical element content (%) C 38 H 24 N 2 O 2 S: C, 79.70; H, 4.22; N, 4.89; S, 5.60. Measured element content (%): C, 79.77; H, 4.20; N, 4.81; S, 5.65.
specific Embodiment 2
[0041]
[0042] Further purification using reverse phase column chromatography with acetonitrile as eluent gave a white solid and its structure was determined by mass spectrometry, HRMS Calcd for C 48 H 36 N 2 O 2 S: 704.25, Found: 704.29. Theoretical element content (%) C 48 H 36 N 2 O 2 S: C, 81.79; H, 5.15; N, 3.97; S, 4.55. Measured element content (%): C, 81.72; H, 5.11; N, 3.91; S, 4.50.
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