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Preparation process for composite of rare earth modified carbon-fibre/polytetrafluoroethylene

A technology of polytetrafluoroethylene and composite materials, which is applied in the field of preparation of rare earth modified carbon fiber/polytetrafluoroethylene composite materials, can solve the problems of poor interfacial bonding force, poor processing performance, and large fiber damage of composite materials, and achieve improved interface Good binding force, low cost and good wear resistance

Inactive Publication Date: 2006-04-12
SHANGHAI JIAOTONG UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

These methods have improved the binding force of the interfacial phase to a certain extent and increased the use value of the composite material, but they have not achieved the desired effect, and there are shortcomings such as unstable effect, easy degradation, large damage to fibers, and poor processability. , resulting in poor interfacial bonding of composite materials

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0023] The raw materials used include: polytetrafluoroethylene, SM021-F type produced by Shanghai Chlor-Alkali Chemical Co., Ltd.; carbon fiber, uncoated polyacrylonitrile-based high-strength type, produced by Jilin Carbon Plant.

[0024] The weight percentages of each component of the rare earth modifier are as follows:

[0025] Lanthanum chloride: 2%, ethanol: 93%, ethylenediaminetetraacetic acid (EDTA): 2%, ammonium chloride: 1%, nitric acid: 0.5%, urea: 1.5%.

[0026] The carbon fiber is pretreated first, and ablated in a muffle furnace at 450°C for 1 hour, so that the residual organic matter on the surface is below 1%. Then, the above-mentioned rare earth modifier was used to treat the carbon fiber in the modifier at room temperature for 2 hours, filtered, and dried.

[0027] The processed carbon fiber is chopped into short fibers of 6 mm, and mixed with the matrix resin by mechanical stirring, the mass percentage of carbon fiber is controlled to be 15% of the mixed powd...

Embodiment 2

[0031] The raw materials used are: polytetrafluoroethylene: SM021-F type produced by Shanghai Chlor-Alkali Chemical Co., Ltd.; carbon fiber: T-300, coated surface treated carbon fiber, produced by Toray Corporation of Japan.

[0032] The weight percentage of each component of the rare earth modifier: 7% of cerium chloride; 76% of ethanol; 9% of ethylenediaminetetraacetic acid (EDTA); 5% of ammonium chloride; 1% of nitric acid; 2% of urea.

[0033] Pre-treat the carbon fiber first, and ablate it in a muffle furnace at 550°C for 0.5 hours, so that the residual organic matter on the surface is below 1%. Then, the above-mentioned rare earth modifier was used to treat the carbon fiber in the modifier at room temperature for 3 hours, filtered, and dried.

[0034] The processed carbon fiber is chopped into short fibers of 10mm, mechanically blended with polytetrafluoroethylene powder, the mass percentage of carbon fiber is 30% of the mixed powder, and then the mixed powder is put int...

Embodiment 3

[0037] The materials are the same as in Example 1, except that the ratio of the rare earth modifier is changed: 10% of lanthanum oxide; 82% of ethanol; 5% of ethylenediaminetetraacetic acid (EDTA); 2% of ammonium chloride; 0.5% of nitric acid;

[0038]The carbon fibers are pretreated first, and ablated in a muffle furnace at 600°C for 0.5 hours, so that the residual organic matter on the surface is below 1%. Then, the above-mentioned rare earth modifier was used to treat the carbon fiber in the modifier at room temperature for 4 hours, filtered, and dried.

[0039] The processed carbon fiber is chopped into short fibers of 15mm, mechanically blended with polytetrafluoroethylene powder, the mass percentage of carbon fiber is 23% of the mixed powder, and then the mixed powder is put into a stainless steel mold for hot pressing , press molding on the press, the pressure is controlled at about 50MPa, and the time is 40 minutes. The process of pressurization and pressure relief is ...

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Abstract

The invention is a method for preparing rare-earth modified fiber / polytetrafluorethylene composite, firstly preprocessing carbon fiber to eliminate surface residual organic substance, adopting rare-earth modifier at room temperature to make surface modifying treatment on the carbon fiber, then cutting the processed carbon fiber short to commix with polytetrafluorethylene powder, and controlling the mass percent of the carbon fiber to the mixture in 15-30%, then, placing the mixture in a stainless steel mould to make hot press moulding, obtaining the composite. The rare-earth modifier is composed of rare-earth compound, alcohol, editic acid, ammonium chloride, nitric acid and urea.

Description

technical field [0001] The invention relates to a method for preparing a composite material, in particular to a method for preparing a rare earth modified carbon fiber / polytetrafluoroethylene composite material, in which carbon fiber (or chopped carbon fiber) treated with a rare earth modifier is filled with polytetrafluoroethylene to prepare a composite material material, in order to improve the bonding force of the interface of carbon fiber / PTFE composite material, and then improve the actual engineering application value of the composite material. Background technique [0002] Carbon fiber reinforced thermoplastic composites have the advantages of strong damage resistance, high elongation at break, good fracture toughness, and low cost. Therefore, thermoplastic composites have become a hot spot in the research and development of resin-based composites. The production technology of carbon fiber reinforced PTFE is relatively mature, the source of raw materials is extensive,...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C08L27/18C08K9/02C08K7/06
Inventor 程先华上官倩芡吴炬
Owner SHANGHAI JIAOTONG UNIV